Cyclotricatechylene based porous crystalline material: Synthesis and applications in gas storage

被引：129

作者：

Yu, Jin-Tao ^{[2
]}

Chen, Zhe ^{[2
]}

Sun, Junliang ^{[1
]}

Huang, Zhi-Tang ^{[2
]}

Zheng, Qi-Yu ^{[2
]}

机构：

[1] Stockholm Univ, Berzelii Ctr EXSELENT Porous Mat, SE-10691 Stockholm, Sweden

[2] Chinese Acad Sci, CAS Key Lab Mol Recognit & Funct, Inst Chem, Beijing Natl Lab Mol Sci, Beijing 100190, Peoples R China

来源：

JOURNAL OF MATERIALS CHEMISTRY | 2012年 / 22卷 / 12期

基金：

中国国家自然科学基金;

关键词：

COVALENT ORGANIC FRAMEWORKS; INTRINSIC MICROPOROSITY; RETICULAR SYNTHESIS; HYDROGEN; CRYPTOPHANES; GENERATION; STABILITY; POLYMERS; CAPACITY; POROSITY;

D O I：

10.1039/c2jm15159f

中图分类号：

O64 [物理化学（理论化学）、化学物理学];

学科分类号：

070304 ; 081704 ;

摘要：

An undulated two-dimensional CTC-based covalent organic framework, CTC-COF, was synthesized through solvothermal reaction for the first time. This mesoporous material stacks in an eclipsed mode in the microcrystalline state. CTC-COF has a surface area of 1710 m(2) g(-1), with a pore width of 2.26 nm calculated by the NL-DFT modelling. The bowl-shaped core unit led to a larger surface area than its analogue, COF-5 constructed by planar subunits. This material has higher low pressure hydrogen uptake than other 2D COFs with similar structures, and even close to the 3D COF materials.

引用

页码：5369 / 5373

页数：5

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