Counterion effects of nickel and sodium dodecylbenzene sulfonate adsorption to multiwalled carbon nanotubes in aqueous solution

被引：208

作者：

Tan, Xiaoli ^{[1
]}

Fang, Ming ^{[2
]}

Chen, Changlun ^{[1
]}

Yu, Shaoming ^{[3
]}

Wang, Xianke ^{[1
]}

机构：

[1] Chinese Acad Sci, Inst Plasma Phys, Hefei 230031, Peoples R China

[2] Chinese Acad Sci, Inst Solid States Phys, Hefei 230031, Peoples R China

[3] Hefei Univ Technol, Coll Chem Engn, Hefei 230009, Peoples R China

来源：

CARBON | 2008年 / 46卷 / 13期

基金：

中国国家自然科学基金;

关键词：

D O I：

10.1016/j.carbon.2008.07.023

中图分类号：

O64 [物理化学（理论化学）、化学物理学];

学科分类号：

070304 ; 081704 ;

摘要：

Batch experiments were conducted to elucidate the adsorption of a widely used anionic surfactant (sodium dodecylbenzene sulfonate (SDBS)) and nickel on multiwalled carbon nanotubes (MWCNTs). Counterion effect on the removal of SDBS and nickel by using MWCNTs was also studied. The microscopic changes of MWCNTs before and after nickel and SDBS adsorption were characterized by scanning electron microscope (SEM) and transmission electron microscope (TEM). X-ray photoelectron spectroscopy (XPS) was performed to study the adsorption mechanism of nickel at a molecular level. The spectroscopic analysis indicated that the adsorption mechanism was mainly attributed to chemical interaction between nickel and the surface functional groups of MWCNTs and surface adsorbed SDBS. The adsorbed SDBS on MWCNTs could lead to the modification of the MWCNT surfaces and partial complexation of nickel with SDBS adsorbed on MWCNTs. MWCNTs are efficient material in the removal of SDBS and nickel from large volume of wastewater. (C) 2008 Elsevier Ltd. All rights reserved.

引用

页码：1741 / 1750

页数：10

共 48 条

[1] An XPS study of the adsorption of lead on goethite (α-FeOOH) [J].

Abdel-Samad, H ;

Watson, PR .

APPLIED SURFACE SCIENCE, 1998, 136 (1-2) :46-54

[2] Removal of anionic surfactant from wastewater by alumina: a case study [J].

Adak, A ;

Bandyopadhyay, M ;

Pal, A .

COLLOIDS AND SURFACES A-PHYSICOCHEMICAL AND ENGINEERING ASPECTS, 2005, 254 (1-3) :165-171

[3] Adsorption studies on Citrus reticulata (fruit peel of orange):: removal and recovery of Ni(II) from electroplating wastewater [J].

Ajmal, M ;

Rao, RAK ;

Ahmad, R ;

Ahmad, J .

JOURNAL OF HAZARDOUS MATERIALS, 2000, 79 (1-2) :117-131

[4] Removal of surfactants by powered activated carbon and microfiltration [J].

Basar, CA ;

Karagunduz, A ;

Cakici, A ;

Keskinler, B .

WATER RESEARCH, 2004, 38 (08) :2117-2124

[5] Kinetics of sodium dodecyl benzene sulfonate adsorption on hematite and its interaction with polyacrylamide [J].

Bhagat, RP .

COLLOID AND POLYMER SCIENCE, 2001, 279 (01) :33-38

[6] Adsorption of Ni(II) from aqueous solution using oxidized multiwall carbon nanotubes [J].

Chen, Changlun ;

Wang, Xiangke .

INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH, 2006, 45 (26) :9144-9149

[7] Extreme oxygen sensitivity of electronic properties of carbon nanotubes [J].

Collins, PG ;

Bradley, K ;

Ishigami, M ;

Zettl, A .

SCIENCE, 2000, 287 (5459) :1801-1804

[8] Biological activity and environmental impact of anionic surfactants [J].

Cserháti, T ;

Forgács, E ;

Oros, G .

ENVIRONMENT INTERNATIONAL, 2002, 28 (05) :337-348

[9] Adsorption isotherm of sodium octylbenzenesulfonate on iron oxide particles in aqueous solutions [J].

Dao, K ;

Bee, A ;

Treiner, C .

JOURNAL OF COLLOID AND INTERFACE SCIENCE, 1998, 204 (01) :61-65

[10] Chromium adsorption by aligned carbon nanotubes supported ceria nanoparticles [J].

Di, ZC ;

Ding, J ;

Peng, XJ ;

Li, YH ;

Luan, ZK ;

Liang, J .

CHEMOSPHERE, 2006, 62 (05) :861-865

← 1 2 3 4 5 →