Impact of mining on the metal content of dust in indigenous villages of northern Chile

被引:34
作者
Zanetta-Colombo, Nicolas C. [1 ,2 ,3 ]
Fleming, Zoe L. [4 ,5 ]
Gayo, Eugenia M. [5 ,6 ]
Manzano, Carlos A. [7 ,8 ]
Panagi, Marios [9 ]
Valdes, Jorge [10 ]
Siegmund, Alexander [1 ,2 ]
机构
[1] Heidelberg Univ, Heidelberg Ctr Environm HCE, Heidelberg, Germany
[2] Heidelberg Univ Educ, Dept Geog, Res Grp Earth Observat Rgeo, Heidelberg, Germany
[3] Heidelberg Univ, Dept Geog, SAI, Heidelberg, Germany
[4] Univ Desarrollo, C Res Ctr Technol Soc, Sch Engn, Envirohlth Dynam Lab, Santiago, Chile
[5] Ctr Climate & Resilience Res CR 2, Santiago, Chile
[6] ANID Millennium Sci Initiat Program Nucleo Mileni, Santiago, Chile
[7] Univ Chile, Fac Ciencias, Dept Quim, Santiago, Chile
[8] San Diego State Univ, Sch Publ Hlth, San Diego, CA 92182 USA
[9] Univ Leicester, Sch Phys & Astron, Leicester, Leics, England
[10] Univ Antofagasta, Lab Sedimentol & Paleoambientes LASPAL, Inst Ciencias Nat Alexander von Humboldt, Fac Ciencias Mar & Recursos Biol, Antofagasta, Chile
关键词
Toxic metal; Mining emissions; Pollution risk; Health risk assessment; Atacama; HEALTH-RISK ASSESSMENT; HEAVY-METALS; ATACAMA DESERT; INDOOR DUST; STREET DUST; ATMOSPHERIC DUST; COPPER DEMAND; MINE; CHUQUICAMATA; SEDIMENTS;
D O I
10.1016/j.envint.2022.107490
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
Indigenous communities from northern Chile have historically been exposed to the impacts of massive copper industrial activities conducted in the region. Some of the communities belonging to the Alto El Loa Indigenous Development Area are located less than 10 km from the "Talabre" tailings dam, which contains residues from copper production and other metals that can be toxic to human health (e.g., As, Sb, Cd, Mo, Pb). Given the increasing demand of copper production to achieve net-zero emission scenarios and concomitant expansions of the tailings, the exposure to toxic metals is a latent risk to local communities. Despite the impact that copper production could generate on ancestral communities from northern Chile, studies and monitoring are limited and the results are often not made accessible for local communities. Here, we evaluate such risks by characterizing metal concentrations in dust collected from roofs and windows of houses from the Alto El Loa area. Our results showed that As, Sb, Cd, Cu, Mo, Ag, S, and Pb concentrations in these matrices can be connected to local copper mining activities. Additionally, air transport models indicate that high concentrations of toxic elements (As, Sb, and Cd) can be explained by the atmospheric transport of particles from the tailings in a NE direction up to 50 km away. Pollution indices and Health Risk Assessment suggested a highly contaminated region with a health risk for its inhabitants. Our analysis on a local scale seeks to make visible the case of northern Chile as a critical territory where actions should be taken to mitigate the effects of mining in the face of this new scenario of in-ternational demand for the raw materials necessary for the transition to a net-zero carbon global society.
引用
收藏
页数:14
相关论文
共 92 条
[81]  
USEPA, 2009, Final Report)
[82]   Environmental problems of illegal gold mining in Madre de Dios (Peru) [J].
Velasquez Zapata, Guadalupe Yahia .
OBSERVATORIO MEDIOAMBIENTAL, 2020, 23 :229-241
[83]  
Vergara Jorge., 2006, Estudios Sociologicos, V24, P331
[84]   Metabolism of arsenic and its toxicological relevance [J].
Watanabe, Takayuki ;
Hirano, Seishiro .
ARCHIVES OF TOXICOLOGY, 2013, 87 (06) :969-979
[85]   The mining sector of Liberia: current practices and environmental challenges [J].
Wilson, Samuel T. K. ;
Wang, Hongtao ;
Kabenge, Martin ;
Qi, Xuejiao .
ENVIRONMENTAL SCIENCE AND POLLUTION RESEARCH, 2017, 24 (23) :18711-18720
[86]   Source Identification and Health Risk Assessment of Metals in Indoor Dust in the Vicinity of Phosphorus Mining, Guizhou Province, China [J].
Yang, Qin ;
Chen, Huaguo ;
Li, Baizhan .
ARCHIVES OF ENVIRONMENTAL CONTAMINATION AND TOXICOLOGY, 2015, 68 (01) :20-30
[87]   Characteristic comparison of heavy metal contamination between road-deposited and roof-deposited sediments in suburban area [J].
Yu, Jianghua ;
Yu, Haixia ;
Xu, Liqiang ;
Tao, Tao ;
Zhang, Yanxing ;
Hua, Yuhao ;
Nkolola, Namwiinga Babra .
ENVIRONMENTAL SCIENCE AND POLLUTION RESEARCH, 2017, 24 (14) :12871-12881
[88]   Hydrochemical and environmental isotope analysis of groundwater and surface water in a dry mountain region in Northern Chile [J].
Zang, Carina ;
Dame, Juliane ;
Nuesser, Marcus .
ENVIRONMENTAL MONITORING AND ASSESSMENT, 2018, 190 (06)
[89]   Risk assessment of potentially toxic elements in smaller than 100-μm street dust particles from a valley-city in northwestern China [J].
Zhao, Ni ;
Lu, Xinwei ;
Chao, Shigang .
ENVIRONMENTAL GEOCHEMISTRY AND HEALTH, 2016, 38 (02) :483-496
[90]   Global anthropogenic atmospheric emission inventory of twelve typical hazardous trace elements, 1995-2012 [J].
Zhu, Chuanyong ;
Tian, Hezhong ;
Hao, Jiming .
ATMOSPHERIC ENVIRONMENT, 2020, 220