An asymmetric naphthalimide derivative for n-channel organic field-effect transistors

被引：13
作者：
Wang, Zongrui [1 ,2 ]
Zhao, Jianfeng [3 ,4 ,5 ]
Dong, Huanli [1 ,6 ]
Qiu, Ge [1 ,6 ]
Zhang, Qichun [3 ,7 ]
Hu, Wenping [1 ]
机构：
[1] Chinese Acad Sci, Inst Chem, Key Lab Organ Solids, Beijing Natl Lab Mol Sci, Beijing 100190, Peoples R China
[2] Univ Chinese Acad Sci, Beijing 100049, Peoples R China
[3] Nanyang Technol Univ, Sch Mat Sci & Engn, Singapore 639798, Singapore
[4] Nanjing Tech Univ, Jiangsu Natl Synergist Innovat Ctr Adv Mat, Key Lab Flexible Elect, Nanjing 211816, Jiangsu, Peoples R China
[5] Nanjing Tech Univ, Jiangsu Natl Synergist Innovat Ctr Adv Mat, Inst Adv Mat, Nanjing 211816, Jiangsu, Peoples R China
[6] Capital Normal Univ, Dept Chem, Beijing 100048, Peoples R China
[7] Nanyang Technol Univ, Sch Phys & Math Sci, Div Chem & Biol Chem, Singapore 63731, Singapore
来源：
PHYSICAL CHEMISTRY CHEMICAL PHYSICS | 2015年 / 17卷 / 40期
基金：
中国国家自然科学基金;
关键词：
HIGH-ELECTRON-MOBILITY; THIN-FILM MORPHOLOGY; HIGH-PERFORMANCE; PHYSICAL-PROPERTIES; SEMICONDUCTORS; POLYMER; MOLECULES; TRANSPORT; THIENOACENE; BEHAVIOR;
D O I：
10.1039/c5cp01302j
中图分类号：
O64 [物理化学（理论化学）、化学物理学];
学科分类号：
070304 ; 081704 ;
摘要：
A new naphthalene diimide (NDI) derivative with an asymmetric aromatic backbone of 2-tetradecylbenzo[lmn]benzo[4,5]imidazo[2,1-b][3,8] phenanthroline-1,3,6(2H)-trione (IZ0) was designed and synthesized. Low LUMO level, large energy gap, and high thermal stability are characterized for this IZ0 compound. The OFET devices based on an IZ0 semiconductor exhibit typical n-type behavior. Through continuously optimizing the fabrication conditions, high performance n-channel OFETs were fabricated based on IZ0 films and single crystals, with the highest carrier mobility of 0.072 cm(2) V-1 s(-1) and 0.22 cm(2) V-1 s(-1), respectively.
引用
收藏
页码：26519 / 26524
页数：6
相关论文
共 50 条
[31]   Asymmetric pyrene derivatives for organic field-effect transistors [J].
Zoephel, Lukas ;
Beckmann, Dirk ;
Enkelmann, Volker ;
Chercka, Dennis ;
Rieger, Ralph ;
Muellen, Klaus .
CHEMICAL COMMUNICATIONS, 2011, 47 (24) :6960-6962
[32]   Polymer binder assisted, solution processed cyanophenyl functionalized diketopyrrolopyrrole microwire for n-channel field-effect transistors [J].
Sim, Kyoseung ;
Palai, Akshaya K. ;
Tarsoly, Gergely ;
Na, Hanah ;
Pyo, Seungmoon .
SYNTHETIC METALS, 2019, 250 :152-160
[33]   Pronounced Side Chain Effects in Triple Bond-Conjugated Polymers Containing Naphthalene Diimides for n-Channel Organic Field-Effect Transistors [J].
Nam, Sungho ;
Hahm, Suk Gyu ;
Khim, Dongyoon ;
Kim, Hwajeong ;
Sajoto, Tissa ;
Ree, Moonhor ;
Marder, Seth R. ;
Anthopoulos, Thomas D. ;
Bradley, Donal D. C. ;
Kim, Youngkyoo .
ACS APPLIED MATERIALS & INTERFACES, 2018, 10 (15) :12921-12929
[34]   Air-Stable n-Channel Organic Single Crystal Field-Effect Transistors Based on Microribbons of Core-Chlorinated Naphthalene Diimide [J].
He, Tao ;
Stolte, Matthias ;
Wuerthner, Frank .
ADVANCED MATERIALS, 2013, 25 (48) :6951-6955
[35]   High performance n-channel organic field-effect transistors based on halogenated derivatives of 1,2,4,5-benzenetetracarboxylic diimides [J].
Peng, Yue ;
Cao, Li ;
Li, Zhefeng .
APPLIED SURFACE SCIENCE, 2017, 420 :355-360
[36]   Quinoidal Oligothiophenes with (Acyl)cyanomethylene Termini: Synthesis, Characterization, Properties, and Solution Processed n-Channel Organic Field-Effect Transistors [J].
Suzuki, Yuki ;
Shimawaki, Masafumi ;
Miyazaki, Eigo ;
Osaka, Itaru ;
Takimiya, Kazuo .
CHEMISTRY OF MATERIALS, 2011, 23 (03) :795-804
[37]   Corannulene derivatives with low LUMO levels and dense convex-concave packing for n-channel organic field-effect transistors [J].
Chen, Rui ;
Lu, Ru-Qiang ;
Shi, Ke ;
Wu, Fan ;
Fang, Hong-Xun ;
Niu, Zhe-Xuan ;
Yan, Xiao-Yun ;
Luo, Ming ;
Wang, Xin-Chang ;
Yang, Chi-Yuan ;
Wang, Xiao-Ye ;
Xu, Binbin ;
Xia, Haiping ;
Pei, Jian ;
Cao, Xiao-Yu .
CHEMICAL COMMUNICATIONS, 2015, 51 (72) :13768-13771
[38]   Low operating voltage n-channel organic field effect transistors using lithium fluoride/PMMA bilayer gate dielectric [J].
Kumar, S. ;
Dhar, A. .
MATERIALS RESEARCH BULLETIN, 2015, 70 :590-594
[39]   ((Alkyloxy)carbonyl)cyanomethylene-Substituted Thienoquinoidal Compounds: a New Class of Soluble n-Channel Organic Semiconductors for Air-Stable Organic Field-Effect Transistors [J].
Suzuki, Yuki ;
Miyazaki, Eigo ;
Takimiya, Kazuo .
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY, 2010, 132 (30) :10453-10466
[40]   New Core-Expanded Naphthalene Diimides for n-Channel Organic Thin Film Transistors [J].
Hu, Yunbin ;
Wang, Zhongli ;
Zhang, Xu ;
Yang, Xiaodi ;
Li, Hongxiang ;
Gao, Xike .
CHINESE JOURNAL OF CHEMISTRY, 2013, 31 (11) :1428-1438
12345