Continuous flow-based laser-assisted plasmonic heating: A new approach for photothermal energy conversion and utilization

被引:27
作者
Belekoukia, Meltiani [1 ]
Kalamaras, Evangelos [1 ]
Tan, Jeannie Z. Y. [1 ]
Vilela, Filipe [3 ]
Garcia, Susana [1 ]
Maroto-Valer, M. Mercedes [1 ]
Xuan, Jin [2 ]
机构
[1] Heriot Watt Univ, Sch Engn & Phys Sci, RCCS, Edinburgh EH14 4AS, Midlothian, Scotland
[2] Loughborough Univ, Dept Chem Engn, Loughborough, Leics, England
[3] Heriot Watt Univ, Sch Engn & Phys Sci, Inst Chem Sci, Edinburgh EH14 4AS, Midlothian, Scotland
基金
英国工程与自然科学研究理事会;
关键词
Plasmonic nanoparticles; Laser irradiation; Photothermal performance; Continuous flow system; SOLAR THERMAL-CONVERSION; DIRECT ABSORPTION; ENHANCED PHOTOCATALYSIS; METAL NANOSTRUCTURES; STEAM-GENERATION; NANOFLUIDS; EFFICIENCY; REDUCTION; SYSTEM; FILMS;
D O I
10.1016/j.apenergy.2019.04.069
中图分类号
TE [石油、天然气工业]; TK [能源与动力工程];
学科分类号
0807 ; 0820 ;
摘要
The aim of this study is to enhance our understanding on photothermal performance of plasmonic Au/TiO2 nanoparticles by conducting a well-controlled experiment under continuous flow conditions. Herein, plasmonic heating experiments of Au nanoparticles decorated on TiO2 nanoparticles were performed using 532 nm laser irradiation. Different parameters, such as Au loading, concentration of nanoparticles, flow rate and laser intensity that could affect the optical and photothermal properties of the nanofluids were studied. The results revealed that the photothermal performance of the nanofluids was remarkably increased in the presence of Au. Particularly, Au nanofluid exhibits a significant higher temperature achieving up to 32 degrees C compared to that of TiO2 nanofluid (22.5 degrees C) and water-based fluid (20.5 degrees C) which is attributed to the localized surface plasmon resonance effect on the surface of Au nanoparticles. The concept of continuous-flow based plasmonic heating of Au/TiO2 nanofluid, with considerable optical and thermal properties, is a promising approach in efficient photothermal applications such as thermal energy supply in industrial chemical processes.
引用
收藏
页码:517 / 524
页数:8
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