The role of mass spectrometry in radioactive contamination assessment after the Fukushima nuclear accident

被引：40

作者：

Bu, Wenting ^{[1
]}

Ni, Youyi ^{[2
,3
]}

Steinhauser, Georg ^{[4
]}

Zheng, Wang ^{[5
]}

Zheng, Jian ^{[2
]}

Furuta, Naoki ^{[6
]}

机构：

[1] China Acad Engn Phys, Inst Nucl Phys & Chem, Mianyang 621900, Peoples R China

[2] Natl Inst Quantum & Radiol Sci & Technol, Fukushima Project Headquarters, Natl Inst Radiol Sci, Inage Ku, Anagawa 4-9-1, Chiba 2638555, Japan

[3] Peking Univ, Sch Phys, State Key Lab Nucl Phys & Technol, Beijing 100871, Peoples R China

[4] Leibniz Univ Hannover, Inst Radioecol & Radiat Protect, D-30419 Hannover, Germany

[5] Arizona State Univ, Sch Earth & Space Explorat, Tempe, AZ 85201 USA

[6] Chuo Univ, Fac Sci & Engn, Dept Appl Chem, Bunkyo Ku, 1-13-27 Kasuga, Tokyo 1128551, Japan

来源：

JOURNAL OF ANALYTICAL ATOMIC SPECTROMETRY | 2018年 / 33卷 / 04期

基金：

中国国家自然科学基金;

关键词：

INDUCTIVELY-COUPLED PLASMA; POWER-PLANT ACCIDENT; CESIUM ISOTOPE COMPOSITIONS; CS-135/CS-137 ATOMIC RATIO; DAIICHI EXCLUSION ZONE; ICP-DRC-MS; ENVIRONMENTAL-SAMPLES; PLUTONIUM ISOTOPES; PU ISOTOPES; SOIL SAMPLES;

D O I：

10.1039/c7ja00401j

中图分类号：

O65 [分析化学];

学科分类号：

070302 ; 081704 ;

摘要：

The Fukushima nuclear accident caused the release of large amounts of radionuclides into the environment. After the accident, radioactive contamination assessment in environmental samples is essential for radiation dose estimation and radioactive remediation. Mass spectrometry characterized by high sensitivity, low detection limit, short measuring time, high sample throughput, and the capability to obtain atomic ratios is a promising technique for the analysis of the accident released long-lived radionuclides. This review describes the developed analytical methods based on mass spectrometric techniques for the determination of radionuclides (Pu isotopes, U isotopes, radiocesium, radioiodine, radiostrontium, etc.) with regards to Fukushima samples. The real applications of mass spectrometric techniques for radioactive source identification, radiation protection and geochemical tracing are discussed to highlight the importance of mass spectrometric techniques in radioactive contamination assessment after the accident. Future research prospects of mass spectrometric techniques for the analysis of radionuclides with application to Fukushima samples are briefly outlined.

引用

页码：519 / 546

页数：28

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