Persistence, temporal and spatial profiles of ultraviolet absorbents and phenolic personal care products in riverine and estuarine sediment of the Pearl River catchment, China

被引：102

作者：

Peng, Xianzhi ^{[1
,3
]}

Xiong, Songsong ^{[1
,2
,3
]}

Ou, Weihui ^{[1
,2
]}

Wang, Zhifang ^{[1
,2
]}

Tan, Jianhua ^{[4
]}

Jin, Jiabin ^{[1
,2
,3
]}

Tang, Caiming ^{[1
,2
]}

Liu, Jun ^{[1
,2
,3
]}

Fan, Yujuan ^{[1
,2
,3
]}

机构：

[1] Chinese Acad Sci, Guangzhou Inst Geochem, State Key Lab Organ Geochem, Guangzhou 510640, Guangdong, Peoples R China

[2] Univ Chinese Acad Sci, Beijing 100049, Peoples R China

[3] Prov Key Lab Environm Utilizat & Protect Guangdon, Guangzhou 510640, Guangdong, Peoples R China

[4] Guangzhou Inst Qual Monitoring & Inspect, Guangzhou 510110, Guangdong, Peoples R China

来源：

JOURNAL OF HAZARDOUS MATERIALS | 2017年 / 323卷

基金：

中国国家自然科学基金;

关键词：

Emerging contaminants; Ultraviolet absorbents; Personal care products; Sediment record; Pearl river catchment; WATER TREATMENT PLANTS; ECOLOGICAL RISK-ASSESSMENT; UV-FILTERS; WASTE-WATER; SURFACE WATERS; UNITED-STATES; IN-VITRO; ANTIMICROBIALS TRICLOCARBAN; WIDESPREAD OCCURRENCE; DIOXIN PHOTOPRODUCTS;

D O I：

10.1016/j.jhazmat.2016.05.020

中图分类号：

X [环境科学、安全科学];

学科分类号：

08 ; 0830 ;

摘要：

A variety of personal care products have been classified as emerging contaminants (ECs). Occurrence, fate, spatial and vertical profiles of 13 ultraviolet absorbents, triclocarban (TCC) and its dechlorinated products, triclosan (TCS), 2-phenylphenol and parabens were investigated in riverine and estuarine sediment of the Pearl River catchment, China. Bisphenol A (BPA), a widely applied plasticizer, was also investigated. The ECs were widely present in the bed sediment. TCC was the most abundant with a maximum concentration of 332 ng g(-1) dry weight. The other prominent ECs included BPA, TCS, octocrylene, and benzotriazole UV stabilizers UV326 and UV328. Treated wastewater effluent was the major source of the ECs in the riverine sediment. TCC, BPA, TCS, methyparaben, UV531, UV326, and UV328 were also detected throughout the estuarine sediment cores, indicating their persistence in the sediment. Temporal trends of the ECs in the sediment cores reflected a combined effect of industrial development, population growth, human life quality improvement, and waste treatment capacity in the Pearl River Delta over the last decades. TCC dechlorination products were frequently detected in the bed sediment with higher levels near treated effluent outlets but only occasionally observed in the sediment cores, suggesting insignificant in-situ TCC dechlorination in the sediment. (C) 2016 Elsevier B.V. All rights reserved.

引用

页码：139 / 146

页数：8

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