Fabrication and photocatalytic properties of flexible g-C3N4/SiO2 composite membrane by electrospinning method

被引:42
作者
Chang, Meng-Jie [1 ,2 ]
Cui, Wen-Na [1 ]
Liu, Jun [1 ]
Wang, Kang [1 ]
Chai, Xiao-Jiao [1 ]
机构
[1] Xian Univ Sci & Technol, Dept Mat Sci & Engn, Xian 710054, Shaanxi, Peoples R China
[2] Shaanxi Normal Univ, Sch Chem & Chem Engn, Xian 710062, Shaanxi, Peoples R China
基金
中国国家自然科学基金;
关键词
ELECTROCATALYSTS; NANOFIBERS; NANOSHEETS; HYBRID;
D O I
10.1007/s10854-018-8663-6
中图分类号
TM [电工技术]; TN [电子技术、通信技术];
学科分类号
0808 ; 0809 ;
摘要
A novel flexible graphitic carbon nitride loaded SiO2 (g-C3N4/SiO2) nanofibrous membrane was fabricated for photocatalytic degradation of dyes. The g-C3N4 nanosheets were directly grown on the electrospun SiO2 nanofiber surface by thermal condensation of urea precursor. X-ray photoelectron spectroscopy and Fourier-transform infrared spectroscopy detections confirmed the successful preparation of the g-C3N4 nanosheets. The g-C3N4 nanosheets with a few layers in thickness were tightly attached on the SiO2 nanofiber surface. The obtained g-C3N4/SiO2 catalysts exhibited high catalytic performance towards decomposition of Rhodamine B under visible light irradiation. The photocatalytic activity remained above 90% within 80 min illumination even after five cycles. Due to the easy preparation and high photocatalytic performance, as well as convenient collection for reuse, the obtained g-C3N4/SiO2 hybrid membranes are promising catalysts for practical application.
引用
收藏
页码:6771 / 6778
页数:8
相关论文
共 35 条
[1]  
Baker BM, 2015, NAT MATER, V14, P1262, DOI [10.1038/NMAT4444, 10.1038/nmat4444]
[2]   Polymeric Photocatalysts Based on Graphitic Carbon Nitride [J].
Cao, Shaowen ;
Low, Jingxiang ;
Yu, Jiaguo ;
Jaroniec, Mietek .
ADVANCED MATERIALS, 2015, 27 (13) :2150-2176
[3]   Facile preparation of novel Fe2O3/BiOI hybrid nanostructures for efficient visible light photocatalysis [J].
Chang, Meng-Jie ;
Wang, Hua ;
Li, Hui-Lu ;
Liu, Jun ;
Du, Hui-Ling .
JOURNAL OF MATERIALS SCIENCE, 2018, 53 (05) :3682-3691
[4]   Experimental Research on Longitudinal Steel Bar Bond Properties in Modified Recycled Aggregate Concrete Beam-Column Interior Joint under Cyclic Loading [J].
Fu, Jia-Li ;
Liu, Bing-Kang ;
Ma, Jun-Wei .
ADVANCES IN MATERIALS SCIENCE AND ENGINEERING, 2017, 2017
[5]   Single Atom (Pd/Pt) Supported on Graphitic Carbon Nitride as an Efficient Photocatalyst for Visible-Light Reduction of Carbon Dioxide [J].
Gao, Guoping ;
Jiao, Yan ;
Waclawik, Eric R. ;
Du, Aijun .
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY, 2016, 138 (19) :6292-6297
[6]   Functional carbon nitride materials design strategies for electrochemical devices [J].
Kessler, Fabian K. ;
Zheng, Yun ;
Schwarz, Dana ;
Merschjann, Christoph ;
Schnick, Wolfgang ;
Wang, Xinchen ;
Bojdys, Michael J. .
NATURE REVIEWS MATERIALS, 2017, 2 (06)
[7]   Nature-Inspired, Highly Durable CO2 Reduction System Consisting of a Binuclear Ruthenium(II) Complex and an Organic Semiconductor Using Visible Light [J].
Kuriki, Ryo ;
Matsunaga, Hironori ;
Nakashima, Takuya ;
Wada, Keisuke ;
Yamakata, Akira ;
Ishitani, Osamu ;
Maeda, Kazuhiko .
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY, 2016, 138 (15) :5159-5170
[8]   Monoclinic Porous BiVO4 Networks Decorated by Discrete g-C3N4 Nano-Islands with Tunable Coverage for Highly Efficient Photocatalysis [J].
Li, Changjiang ;
Wang, Shengping ;
Wang, Tuo ;
Wei, Yijia ;
Zhang, Peng ;
Gong, Jinlong .
SMALL, 2014, 10 (14) :2783-2790
[9]   Pie-like electrode design for high-energy density lithium-sulfur batteries [J].
Li, Zhen ;
Zhang, Jin Tao ;
Chen, Yu Ming ;
Li, Ju ;
Lou, Xiong Wen .
NATURE COMMUNICATIONS, 2015, 6
[10]   Unique Electronic Structure Induced High Photoreactivity of Sulfur-Doped Graphitic C3N4 [J].
Liu, Gang ;
Niu, Ping ;
Sun, Chenghua ;
Smith, Sean C. ;
Chen, Zhigang ;
Lu, Gao Qing ;
Cheng, Hui-Ming .
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY, 2010, 132 (33) :11642-11648