A strategy for the diversity-oriented synthesis of macrocyclic scaffolds using multidimensional coupling

被引:0
作者
Beckmann, Henning S. G. [1 ]
Nie, Feilin [1 ]
Hagerman, Caroline E. [1 ]
Johansson, Henrik [1 ,2 ]
Tan, Yaw Sing [1 ]
Wilcke, David [1 ]
Spring, David R. [1 ]
机构
[1] Univ Cambridge, Dept Chem, Cambridge CB2 1EW, England
[2] Univ Copenhagen, Dept Drug Design & Pharmacol, DK-2100 Copenhagen, Denmark
基金
英国生物技术与生命科学研究理事会; 英国医学研究理事会; 英国工程与自然科学研究理事会; 英国惠康基金;
关键词
SMALL MOLECULES; SOLID-PHASE; DISCOVERY; CYCLOADDITION; CYCLODEXTRIN; EXPLORATION; ALKYNES; AZIDES; RINGS;
D O I
10.1038/NCHEM.1729
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
A prerequisite for successful screening campaigns in drug discovery or chemical genetics is the availability of structurally and thus functionally diverse compound libraries. Diversity-oriented synthesis (DOS) provides strategies for the generation of such libraries, of which the build/couple/pair (B/C/P) algorithm is the most frequently used. We have developed an advanced B/C/P strategy that incorporates multidimensional coupling. In this approach, structural diversity is not only defined by the nature of the building blocks employed, but also by the linking motif installed during the coupling reaction. We applied this step-efficient approach in a DOS of a library that consisted of 73 macrocyclic compounds based around 59 discrete scaffolds. The macrocycles prepared cover a broad range of different molecular shapes, as illustrated by principal moment-of-inertia analysis. This demonstrates the capability of the advanced B/C/P strategy using multidimensional coupling for the preparation of structurally diverse compound collections.
引用
收藏
页码:861 / 867
页数:7
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