High quality ultrathin Bi2Se3 films on CaF2 and CaF2/Si by molecular beam epitaxy with a radio frequency cracker cell

被引:21
作者
Zhang, Li [1 ,2 ]
Hammond, Robert [2 ]
Dolev, Merav [1 ,2 ]
Liu, Min [2 ,3 ]
Palevski, Alexander [4 ]
Kapitulnik, Aharon [1 ,2 ,3 ]
机构
[1] Stanford Univ, Dept Appl Phys, Stanford, CA 94305 USA
[2] Stanford Univ, Geballe Lab Adv Mat, Stanford, CA 94305 USA
[3] Stanford Univ, Dept Phys, Stanford, CA 94305 USA
[4] Tel Aviv Univ, Sch Phys & Astron, IL-69978 Tel Aviv, Israel
关键词
TOPOLOGICAL INSULATORS;
D O I
10.1063/1.4758466
中图分类号
O59 [应用物理学];
学科分类号
摘要
We report a method to fabricate high quality Bi2Se3 thin films using molecular beam epitaxy with a radio frequency cracker cell as an atomic selenium source. With Se-to-Bi ratios close to exact stoichiometry, optimal layer-by-layer growth of high quality Bi2Se3 thin films with smooth surfaces has been achieved on CaF2(111) substrates and Si(111) substrates with a thin epitaxial CaF2 buffer layer (CaF2/Si). Transport measurements show a characteristic weak-antilocalization magnetoresistance in all the films, with the emergence of a weak-localization contribution in the ultrathin film limit. Quantum oscillations, attributed to the topological surface states have been observed, including in films grown on CaF2/Si. (C) 2012 American Institute of Physics. [http://dx.doi.org/10.1063/1.4758466]
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页数:4
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