Controlling the conductivity of amorphous LaAlO3/SrTiO3 interfaces by in-situ application of an electric field during fabrication

被引:12
作者
Trier, F. [1 ]
Amoruso, S. [2 ,3 ]
Christensen, D. V. [1 ]
Sambri, A. [2 ,3 ]
Chen, Y. Z. [1 ]
Wang, X. [2 ,3 ]
Stamate, E. [1 ]
Bruzzese, R. [2 ,3 ]
Pryds, N. [1 ]
机构
[1] Tech Univ Denmark, Dept Energy Convers & Storage, DK-4000 Roskilde, Denmark
[2] CNR SPIN, I-80125 Naples, Italy
[3] Complesso Univ Monte St Angelo, Dipartimento Sci Fis, I-80125 Naples, Italy
关键词
PULSED-LASER DEPOSITION; THIN-FILMS; OXIDE; TEMPERATURE; GAS;
D O I
10.1063/1.4815989
中图分类号
O59 [应用物理学];
学科分类号
摘要
Amorphous-LaAlO3/SrTiO3 interfaces present metallic conductivity similar to those found in their all-crystalline counterparts. Here, the conductivity of amorphous-LaAlO3/SrTiO3 interfaces is modified by an external electric field applied in-situ with a biased truncated cone electrode (-10 V <= V-bias <= 20 V) during film growth. By modulating the charge balance of the arriving plasma species, interfacial conduction of the amorphous-LaAlO3/SrTiO3 heterostructures shifts from metallic to insulating via a semiconducting-like characteristic transport mode. This remarkable behavior is explained by a modification of the Al-ion flux impinging the SrTiO3 surface, which alters the amount of near-interface oxygen vacancies being formed at the SrTiO3 surface. (C) 2013 AIP Publishing LLC.
引用
收藏
页数:5
相关论文
共 31 条
  • [1] Critical influence of target-to-substrate distance on conductive properties of LaGaO3/SrTiO3 interfaces deposited at 10-1 mbar oxygen pressure
    Aruta, C.
    Amoruso, S.
    Ausanio, G.
    Bruzzese, R.
    Di Gennaro, E.
    Lanzano, M.
    Granozio, F. Miletto
    Riaz, Muhammad
    Sambri, A.
    di Uccio, U. Scotti
    Wang, X.
    [J]. APPLIED PHYSICS LETTERS, 2012, 101 (03)
  • [2] Pulsed laser deposition of SrTiO3/LaGaO3 and SrTiO3/LaAlO3: Plasma plume effects
    Aruta, C.
    Amoruso, S.
    Bruzzese, R.
    Wang, X.
    Maccariello, D.
    Granozio, F. Miletto
    di Uccio, U. Scotti
    [J]. APPLIED PHYSICS LETTERS, 2010, 97 (25)
  • [3] Electric field control of the LaAlO3/SrTiO3 interface ground state
    Caviglia, A. D.
    Gariglio, S.
    Reyren, N.
    Jaccard, D.
    Schneider, T.
    Gabay, M.
    Thiel, S.
    Hammerl, G.
    Mannhart, J.
    Triscone, J. -M.
    [J]. NATURE, 2008, 456 (7222) : 624 - 627
  • [4] Nanoscale control of an interfacial metal-insulator transition at room temperature
    Cen, C.
    Thiel, S.
    Hammerl, G.
    Schneider, C. W.
    Andersen, K. E.
    Hellberg, C. S.
    Mannhart, J.
    Levy, J.
    [J]. NATURE MATERIALS, 2008, 7 (04) : 298 - 302
  • [5] Oxide Nanoelectronics on Demand
    Cen, Cheng
    Thiel, Stefan
    Mannhart, Jochen
    Levy, Jeremy
    [J]. SCIENCE, 2009, 323 (5917) : 1026 - 1030
  • [6] A high-mobility two-dimensional electron gas at the spinel/perovskite interface of γ-Al2O3/SrTiO3
    Chen, Y. Z.
    Bovet, N.
    Trier, F.
    Christensen, D. V.
    Qu, F. M.
    Andersen, N. H.
    Kasama, T.
    Zhang, W.
    Giraud, R.
    Dufouleur, J.
    Jespersen, T. S.
    Sun, J. R.
    Smith, A.
    Nygard, J.
    Lu, L.
    Buechner, B.
    Shen, B. G.
    Linderoth, S.
    Pryds, N.
    [J]. NATURE COMMUNICATIONS, 2013, 4
  • [7] Charge modulated interfacial conductivity in SrTiO3-based oxide heterostructures
    Chen, Y. Z.
    Stamate, E.
    Pryds, N.
    Sun, J. R.
    Shen, B. G.
    Linderoth, S.
    [J]. APPLIED PHYSICS LETTERS, 2011, 98 (23)
  • [8] Resistance switching at the interface of LaAlO3/SrTiO3
    Chen, Y. Z.
    Zhao, J. L.
    Sun, J. R.
    Pryds, N.
    Shen, B. G.
    [J]. APPLIED PHYSICS LETTERS, 2010, 97 (12)
  • [9] Metallic and Insulating Interfaces of Amorphous SrTiO3-Based Oxide Heterostructures
    Chen, Yunzhong
    Pryds, Nini
    Kleibeuker, Josee E.
    Koster, Gertjan
    Sun, Jirong
    Stamate, Eugen
    Shen, Baogen
    Rijnders, Guus
    Linderoth, Soren
    [J]. NANO LETTERS, 2011, 11 (09) : 3774 - 3778
  • [10] Controlling interfacial states in amorphous/crystalline LaAlO3/SrTiO3 heterostructures by electric fields
    Christensen, D. V.
    Trier, F.
    Chen, Y. Z.
    Smith, A.
    Nygard, J.
    Pryds, N.
    [J]. APPLIED PHYSICS LETTERS, 2013, 102 (02)