Gasification of coal and biomass as a net carbon-negative power source for environment-friendly electricity generation in China

被引:107
作者
Lu, Xi [1 ,2 ]
Cao, Liang [1 ,2 ,3 ]
Wang, Haikun [4 ]
Peng, Wei [5 ,6 ]
Xing, Jia [1 ,2 ]
Wang, Shuxiao [1 ,2 ]
Cai, Siyi [1 ,2 ]
Shen, Bo [7 ]
Yang, Qing [8 ,9 ,10 ]
Nielsen, Chris P. [10 ]
McElroy, Michael B. [10 ,11 ]
机构
[1] Tsinghua Univ, Sch Environm, State Key Joint Lab Environm Simulat & Pollut Con, Beijing 10084, Peoples R China
[2] Tsinghua Univ, State Environm Protect Key Lab Sources & Control, Beijing 10084, Peoples R China
[3] Univ Queensland, Sch Chem Engn, Brisbane, Qld 4072, Australia
[4] Nanjing Univ, Sch Environm, State Key Lab Pollut Control & Resource Reuse, Nanjing 210023, Jiangsu, Peoples R China
[5] Penn State Univ, Sch Int Affairs, University Pk, PA 16802 USA
[6] Penn State Univ, Dept Civil & Environm Engn, University Pk, PA 16802 USA
[7] Lawrence Berkeley Natl Lab, Energy Anal & Environm Impacts Div, Berkeley, CA 94720 USA
[8] Huazhong Univ Sci & Technol, Sch Energy & Power Engn, Dept New Energy Sci & Technol, Wuhan 430074, Hubei, Peoples R China
[9] Huazhong Univ Sci & Technol, China EU Inst Clean & Renewable Energy, Wuhan 430074, Hubei, Peoples R China
[10] Harvard Univ, John A Paulson Sch Engn & Appl Sci, Cambridge, MA 02138 USA
[11] Harvard Univ, Dept Earth & Planetary Sci, Cambridge, MA 02138 USA
基金
中国国家自然科学基金;
关键词
bioenergy; gasification; CCS; air pollution; carbon-negative energy; ENERGY-CONSUMPTION; GEOLOGICAL STORAGE; CO2; CAPTURE; EMISSIONS; POLLUTANTS; PYROLYSIS; IMPACT; MARKET; TAR; PARTICLES;
D O I
10.1073/pnas.1812239116
中图分类号
O [数理科学和化学]; P [天文学、地球科学]; Q [生物科学]; N [自然科学总论];
学科分类号
07 ; 0710 ; 09 ;
摘要
Realizing the goal of the Paris Agreement to limit global warming to 2 degrees C by the end of this century will most likely require deployment of carbon-negative technologies. It is particularly important that China, as the world's top carbon emitter, avoids being locked into carbon-intensive, coal-fired power-generation technologies and undertakes a smooth transition from high- to negative-carbon electricity production. We focus here on deploying a combination of coal and biomass energy to produce electricity in China using an integrated gasification cycle system combined with carbon capture and storage (CBECCS). Such a system will also reduce air pollutant emissions, thus contributing to China's near-term goal of improving air quality. We evaluate the bus-bar electricity-generation prices for CBECCS with mixing ratios of crop residues varying from 0 to 100%, as well as associated costs for carbon mitigation and cobenefits for air quality. We find that CBECCS systems employing a crop residue ratio of 35% could produce electricity with net-zero life-cycle emissions of greenhouse gases, with a levelized cost of electricity of no more than 9.2 US cents per kilowatt hour. A carbon price of approximately $52.0 per ton would make CBECCS cost-competitive with pulverized coal power plants. Therefore, our results provide critical insights for designing a CBECCS strategy in China to harness near-term air-quality cobenefits while laying the foundation for achieving negative carbon emissions in the long run.
引用
收藏
页码:8206 / 8213
页数:8
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