Optimizing Cs2LiYCl6 for fast neutron spectroscopy

被引:46
作者
D'Olympia, N. [1 ]
Chowdhury, P. [1 ]
Guess, C. J. [1 ]
Harrington, T. [1 ]
Jackson, E. G. [1 ]
Lakshmi, S. [1 ]
Lister, C. J. [1 ]
Glodo, J. [2 ]
Hawrami, R. [2 ]
Shah, K. [2 ]
Shirwadkar, U. [2 ]
机构
[1] Univ Massachusetts, Dept Phys & Appl Phys, Lowell, MA 01854 USA
[2] Radiat Monitoring Devices Inc, Watertown, MA 02472 USA
关键词
Fast neutron detector; CLYC; N-gamma discrimination; Cl-35(nP); Li-6(n alpha); Cs2LiYCl6; SCINTILLATOR;
D O I
10.1016/j.nima.2012.07.021
中图分类号
TH7 [仪器、仪表];
学科分类号
0804 ; 080401 ; 081102 ;
摘要
Cs2UYCl6 (CLYC) has generated recent interest as a thermal neutron detector due to its excellent n/gamma-ray pulse-shape discrimination and energy resolution. Here, the capabilities of CLYC as a fast neutron detector and spectrometer are reported. A 1 in. x 1 in. CLYC detector was used to measure the response of mono-energetic neutrons over a range of 0.8-2.0 MeV produced via the Li-7(p,n) reaction at the University of Massachusetts Lowell 5.5 MV Van de Graaff accelerator. A broad continuum from the Li-6(n, alpha) reaction was observed, as well as additional peaks below the thermal capture peak. Based on possible reactions in CLYC, the additional peaks are determined to be due to the Cl-35(n,p)S-35 reaction, with a Q-value of +615 keV, and corroborated in simulations using MCNPX. The average resolution of 9% for these peaks makes CLYC a promising candidate for a fast neutron spectrometer. Published by Elsevier B.V.
引用
收藏
页码:140 / 146
页数:7
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