Raman-induced Kerr-effect dual-comb spectroscopy

被引：60

作者：

Ideguchi, T. ^{[1
]}

Bernhardt, B. ^{[1
,2
]}

Guelachvili, G. ^{[3
]}

Haensch, T. W. ^{[1
,2
]}

Picque, N. ^{[1
,2
,3
]}

机构：

[1] Max Planck Inst Quantum Opt, D-85748 Garching, Germany

[2] Univ Munich, Fak Phys, D-80799 Munich, Germany

[3] Univ Paris 11, CNRS, Inst Sci Mol Orsay, F-91405 Orsay, France

来源：

OPTICS LETTERS | 2012年 / 37卷 / 21期

基金：

欧洲研究理事会;

关键词：

MICROSCOPY; LASERS;

D O I：

10.1364/OL.37.004498

中图分类号：

O43 [光学];

学科分类号：

070207 ; 0803 ;

摘要：

We report on the first (to our knowledge) demonstration of nonlinear dual-frequency-comb spectroscopy. In multi-heterodyne femtosecond Raman-induced Kerr-effect spectroscopy, the Raman gain resulting from the coherent excitation of molecular vibrations by a spectrally narrow pump is imprinted onto the femtosecond laser frequency comb probe spectrum. The birefringence signal induced by the nonlinear interaction of these beams and the sample is heterodyned against a frequency comb local oscillator with a repetition frequency slightly different from that of the comb probe. Such time-domain interference provides multiplex access to the phase and amplitude Raman spectra over a broad spectral bandwidth within a short measurement time. (C) 2012 Optical Society of America

引用

页码：4498 / 4500

页数：3

共 13 条

[1] Spectroscopy of the methane ν3 band with an accurate midinfrared coherent dual-comb spectrometer [J].

Baumann, E. ;

Giorgetta, F. R. ;

Swann, W. C. ;

Zolot, A. M. ;

Coddington, I. ;

Newbury, N. R. .

PHYSICAL REVIEW A, 2011, 84 (06)

[2] Mid-infrared dual-comb spectroscopy with 2.4 μm Cr2+:ZnSe femtosecond lasers [J].

Bernhardt, B. ;

Sorokin, E. ;

Jacquet, P. ;

Thon, R. ;

Becker, T. ;

Sorokina, I. T. ;

Picque, N. ;

Haensch, T. W. .

APPLIED PHYSICS B-LASERS AND OPTICS, 2010, 100 (01) :3-8

[3] Cavity-enhanced dual-comb spectroscopy [J].

Bernhardt, Birgitta ;

Ozawa, Akira ;

Jacquet, Patrick ;

Jacquey, Marion ;

Kobayashi, Yohei ;

Udem, Thomas ;

Holzwarth, Ronald ;

Guelachvili, Guy ;

Haensch, Theodor W. ;

Picque, Nathalie .

NATURE PHOTONICS, 2010, 4 (01) :55-57

[4] Coherent multiheterodyne spectroscopy using stabilized optical frequency combs [J].

Coddington, Ian ;

Swann, William C. ;

Newbury, Nathan R. .

PHYSICAL REVIEW LETTERS, 2008, 100 (01)

[5] Optical Heterodyne-Detected Raman-Induced Kerr Effect (OHD-RIKE) Microscopy [J].

Freudiger, Christian W. ;

Roeffaers, Maarten B. J. ;

Zhang, Xu ;

Saar, Brian G. ;

Min, Wei ;

Xie, X. Sunney .

JOURNAL OF PHYSICAL CHEMISTRY B, 2011, 115 (18) :5574-5581

[6] Highly specific label-free molecular imaging with spectrally tailored excitation-stimulated Raman scattering (STE-SRS) microscopy [J].

Freudiger, Christian W. ;

Min, Wei ;

Holtom, Gary R. ;

Xu, Bingwei ;

Dantus, Marcos ;

Xie, X. Sunney .

NATURE PHOTONICS, 2011, 5 (02) :103-109

[7] Nobel Lecture:: Passion for precision [J].

Haensch, Theodor W. .

REVIEWS OF MODERN PHYSICS, 2006, 78 (04) :1297-1309

[8]

Ideguchi T., 2012, ARXIV12014177

[9] Synchronization of two passively mode-locked, picosecond lasers within 20 fs for coherent anti-Stokes Raman scattering microscopy [J].

Jones, DJ ;

Potma, EO ;

Cheng, JX ;

Burfeindt, B ;

Pang, Y ;

Ye, J ;

Xie, XS .

REVIEW OF SCIENTIFIC INSTRUMENTS, 2002, 73 (08) :2843-2848

[10] A 75 MHz Light Source for Femtosecond Stimulated Raman Microscopy [J].

Ploetz, E. ;

Marx, B. ;

Klein, T. ;

Huber, R. ;

Gilch, P. .

OPTICS EXPRESS, 2009, 17 (21) :18612-18620

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