New Tricks for Old Molecules: Development and Application of Porous N-doped, Carbonaceous Membranes for CO2 Separation

被引：65

作者：

Zhu, Xiang ^{[1
,2
,3
]}

Tian, Chengcheng ^{[1
,2
,3
]}

Chai, Songhai ^{[3
]}

Nelson, Kimberly ^{[4
]}

Han, Kee Sung ^{[3
]}

Hagaman, Edward W. ^{[3
]}

Veith, Gabriel M. ^{[5
]}

Mahurin, Shannon M. ^{[3
]}

Liu, Honglai ^{[1
,2
]}

Dai, Sheng ^{[3
,4
]}

机构：

[1] E China Univ Sci & Technol, State Key Lab Chem Engn, Shanghai 200237, Peoples R China

[2] E China Univ Sci & Technol, Dept Chem, Shanghai 200237, Peoples R China

[3] Oak Ridge Natl Lab, Div Chem Sci, Oak Ridge, TN 37831 USA

[4] Univ Tennessee, Dept Chem, Knoxville, TN 37996 USA

[5] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA

来源：

ADVANCED MATERIALS | 2013年 / 25卷 / 30期

基金：

中国国家自然科学基金;

关键词：

trimerization of acetyl groups; N-doped membrane; CO2; separation; TRIAZINE-BASED FRAMEWORKS; ORGANIC FRAMEWORKS; HIGH PERMEABILITY; ACTIVATED CARBON; SIEVE STRUCTURE; POLYMER; PERFORMANCE; COVALENT; TRANSPORT; CAPTURE;

D O I：

10.1002/adma.201300793

中图分类号：

O6 [化学];

学科分类号：

0703 ;

摘要：

A new strategy is successfully applied to "old" acetyl compounds. A free-standing, porous, N-doped carbonaceous membrane is facilely prepared from the thermal treatment of a pyrrole-ring-containing polymeric membrane based on the superacid-catalyzed copolymerization of acetyl monomers. An exceptional ideal CO2/N2 permselectivity of 43.2 is achieved with a good CO2 permeability of 1149.3 Barrer, exceeding the recent upper bound for CO2/N2. Copyright © 2013 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim.

引用

页码：4152 / 4158

页数：7

共 64 条

[1]

[Anonymous], 2013, Angew Chem, DOI 10.1002/ange.201206339

[2] A High-Performance Gas-Separation Membrane Containing Submicrometer-Sized Metal-Organic Framework Crystals [J].

Bae, Tae-Hyun ;

Lee, Jong Suk ;

Qiu, Wulin ;

Koros, William J. ;

Jones, Christopher W. ;

Nair, Sankar .

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION, 2010, 49 (51) :9863-9866

[3] Facile High-Yield Solvothermal Deposition of Inorganic Nanostructures on Zeolite Crystals for Mixed Matrix Membrane Fabrication [J].

Bae, Tae-Hyun ;

Liu, Junqiang ;

Lee, Jong Suk ;

Koros, William J. ;

Jones, Christopher W. ;

Nair, Sankar .

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY, 2009, 131 (41) :14662-+

[4] Natural gas processing with membranes: An overview [J].

Baker, Richard W. ;

Lokhandwala, Kaaeid .

INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH, 2008, 47 (07) :2109-2121

[5] Room-Temperature Ionic Liquids and Composite Materials: Platform Technologies for CO2 Capture [J].

Bara, Jason E. ;

Camper, Dean E. ;

Gin, Douglas L. ;

Noble, Richard D. .

ACCOUNTS OF CHEMICAL RESEARCH, 2010, 43 (01) :152-159

[6] Polymer-Supported and Free-Standing Metal-Organic Framework Membrane [J].

Ben, Teng ;

Lu, Chunjing ;

Pei, Cuiying ;

Xu, Shixian ;

Qiu, Shilun .

CHEMISTRY-A EUROPEAN JOURNAL, 2012, 18 (33) :10250-10253

[7] Rational Extension of the Family of Layered, Covalent, Triazine-Based Frameworks with Regular Porosity [J].

Bojdys, Michael J. ;

Jeromenok, Jekaterina ;

Thomas, Arne ;

Antonietti, Markus .

ADVANCED MATERIALS, 2010, 22 (19) :2202-+

[8]

Bunck D. N., 2012, ANGEW CHEM, V124, P1921, DOI [10.1002/ange.201108462, DOI 10.1021/acs.chemrev.9b00550]

[9] Internal Functionalization of Three-Dimensional Covalent Organic Frameworks [J].

Bunck, David N. ;

Dichtel, William R. .

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION, 2012, 51 (08) :1885-1889

[10] Nanoporous Organic Polymer/Cage Composite Membranes [J].

Bushell, Alexandra F. ;

Budd, Peter M. ;

Attfield, Martin P. ;

Jones, James T. A. ;

Hasell, Tom ;

Cooper, Andrew I. ;

Bernardo, Paola ;

Bazzarelli, Fabio ;

Clarizia, Gabriele ;

Jansen, Johannes C. .

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION, 2013, 52 (04) :1253-1256

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