Green Chemistry Approach to Surface Decoration: Trimesic Acid Self-Assembly on HOPG

被引：24
|
作者：
Korolkov, Vladimir V. [1 ]
Allen, Stephanie [1 ]
Roberts, Clive J. [1 ]
Tendler, Saul J. B. [1 ]
机构：
[1] Univ Nottingham, Sch Pharm, Lab Biophys & Surface Anal, Nottingham NG7 2RD, England
来源：
JOURNAL OF PHYSICAL CHEMISTRY C | 2012年 / 116卷 / 21期
关键词：
2-DIMENSIONAL MOLECULAR NETWORK; LIQUID-SOLID INTERFACE; CYANURIC ACID; COORDINATION NETWORKS; HYDROGEN; MELAMINE; AU(111); ADSORPTION; MONOLAYERS;
D O I：
10.1021/jp212388c
中图分类号：
O64 [物理化学（理论化学）、化学物理学];
学科分类号：
070304 ; 081704 ;
摘要：
We have investigated trimesic acid (1,3,5-benzenetricarboxylic acid, TMA) adsorption on highly oriented pyrolytic graphite (HOPG) surface from aqueous medium at room temperature. Both atomic force microscopy and scanning tunneling microscopy were utilized to follow the adsorption dynamics and molecular arrangements. We have proposed an optimized green chemistry approach for fabricating trimesic acid monolayer structures on HOPG. A chicken-wire arrangement for adsorbed molecules with an average pore size of 11 +/- 1 angstrom was established and was observed using both scanning techniques. This structure was found to be stable in the ambient for at least two days.
引用
收藏
页码：11519 / 11525
页数：7
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