Multifarious roles of carbon quantum dots in heterogeneous photocatalysis

被引:128
作者
Lu, Kang-Qiang [1 ,2 ]
Quan, Quan [1 ,2 ]
Zhang, Nan [1 ,2 ]
Xu, Yi-Jun [1 ,2 ]
机构
[1] Fuzhou Univ, Coll Chem, State Key Lab Photocatalysis Energy & Environm, Fuzhou 350002, Fujian, Peoples R China
[2] Fuzhou Univ, Coll Chem, New Campus, Fuzhou 350108, Fujian, Peoples R China
基金
中国国家自然科学基金;
关键词
Carbon quantum dots; Multifarious roles; Photocatalysis applications; Solar energy conversion; VISIBLE-LIGHT IRRADIATION; NEAR-INFRARED IRRADIATION; SOLAR-ENERGY CONVERSION; UP-CONVERSION; ULTRASONIC PREPARATION; EMERGENT NANOLIGHTS; HYBRID NANOSHEETS; NICKEL-CATALYST; GRAPHENE; COMPOSITES;
D O I
10.1016/j.jechem.2016.09.015
中图分类号
O69 [应用化学];
学科分类号
081704 ;
摘要
As a new member of carbon material family, carbon quantum dots (CQDs) have attracted tremendous attentions for their potentials in the heterogeneous photocatalysis applications. Due to the unique microstructure and optical properties, the roles of CQDs played in the CQDs-based photocatalytic systems have been found to be diverse with the continuous researches in this regard. Herein, we provide a concise minireview to elaborate the multifarious roles of CQDs in photocatalysis, including photoelectron mediator and acceptor, photosensitizer, photocatalyst, reducing agent for metal salt, enhancing adsorption capacity and spectral converter. In addition, the perspectives on future research trends and challenges are proposed, which are anticipated to stimulate further research into this promising field on designing a variety of efficient CQDs-based photocatalysts for solar energy conversion. (C) 2016 Science Press and Dalian Institute of Chemical Physics, Chinese Academy of Sciences. Published by Elsevier B. V. and Science Press. All rights reserved.
引用
收藏
页码:927 / 935
页数:9
相关论文
共 94 条
[1]   The design and development of highly reactive titanium oxide photocatalysts operating under visible light irradiation [J].
Anpo, M ;
Takeuchi, M .
JOURNAL OF CATALYSIS, 2003, 216 (1-2) :505-516
[2]   Visible Photocatalytic Activity Enhancement of ZnWO4 by Graphene Hybridization [J].
Bai, Xiaojuan ;
Wang, Li ;
Zhu, Yongfa .
ACS CATALYSIS, 2012, 2 (12) :2769-2778
[3]   Luminescent Carbon Nanodots: Emergent Nanolights [J].
Baker, Sheila N. ;
Baker, Gary A. .
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION, 2010, 49 (38) :6726-6744
[4]   A misunderstanding about upconversion luminescence of carbon quantum dots [J].
Barati, Ali ;
Shamsipur, Mojtaba ;
Abdollahi, Hamid .
JOURNAL OF THE IRANIAN CHEMICAL SOCIETY, 2015, 12 (03) :441-446
[5]   Carbon dots for multiphoton bioimaging [J].
Cao, Li ;
Wang, Xin ;
Meziani, Mohammed J. ;
Lu, Fushen ;
Wang, Haifang ;
Luo, Pengju G. ;
Lin, Yi ;
Harruff, Barbara A. ;
Veca, L. Monica ;
Murray, Davoy ;
Xie, Su-Yuan ;
Sun, Ya-Ping .
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY, 2007, 129 (37) :11318-+
[6]   Carbon Nanoparticles as Visible-Light Photocatalysts for Efficient CO2 Conversion and Beyond [J].
Cao, Li ;
Sahu, Sushant ;
Anilkumar, Parambath ;
Bunker, Christopher E. ;
Xu, Juan ;
Fernando, K. A. Shiral ;
Wang, Ping ;
Guliants, Elena A. ;
Tackett, Kenneth N., II ;
Sun, Ya-Ping .
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY, 2011, 133 (13) :4754-4757
[7]   Well-controlled layer-by-layer assembly of carbon dot/CdS heterojunctions for efficient visible-light-driven photocatalysis [J].
Chai, Na-Na ;
Wang, Hang-Xing ;
Hu, Chen-Xia ;
Wang, Qiang ;
Zhang, Hao-Li .
JOURNAL OF MATERIALS CHEMISTRY A, 2015, 3 (32) :16613-16620
[8]   Photocatalytic construction and building materials: From fundamentals to applications [J].
Chen, Jun ;
Poon, Chi-sun .
BUILDING AND ENVIRONMENT, 2009, 44 (09) :1899-1906
[9]   Heterogeneous photocatalytic nanomaterials: prospects and challenges in selective transformations of biomass-derived compounds [J].
Colmenares, Juan Carlos ;
Luque, Rafael .
CHEMICAL SOCIETY REVIEWS, 2014, 43 (03) :765-778
[10]   The synergistic role of carbon quantum dots for the improved photocatalytic performance of Bi2MoO6 [J].
Di, Jun ;
Xia, Jiexiang ;
Ji, Mengxia ;
Li, Hongping ;
Xu, Hui ;
Li, Huaming ;
Chen, Rong .
NANOSCALE, 2015, 7 (26) :11433-11443