Two-dimensional electronic spectroscopy for mapping molecular photophysics

被引：24

作者：

Anna, Jessica M. ^{[1
]}

Song, Yin ^{[1
]}

Dinshaw, Rayomond ^{[1
]}

Scholes, Gregory D. ^{[1
]}

机构：

[1] Univ Toronto, Dept Chem, Toronto, ON M5S 3H6, Canada

来源：

PURE AND APPLIED CHEMISTRY | 2013年 / 85卷 / 07期

基金：

加拿大自然科学与工程研究理事会;

关键词：

energy transfer; light harvesting; molecular aggregates; phasing; photosynthesis; two-dimensional electronic spectroscopy; ultrafast spectroscopy; PHOTOSYSTEM-I; ENERGY-TRANSFER; QUANTUM COHERENCE; SPECTRAL INTERFEROMETRY; OPTICAL SPECTROSCOPY; TRANSIENT ABSORPTION; CHARGE SEPARATION; PHASE; FLUORESCENCE; DYNAMICS;

D O I：

10.1351/PAC-CON-12-10-21

中图分类号：

O6 [化学];

学科分类号：

0703 ;

摘要：

We demonstrate the ability of two-dimensional electronic spectroscopy (2DES) to map ultrafast energy transfer and dynamics in two systems: the pigment-protein complex photosystem I (PSI) and aggregates of the conjugated polymer poly(3-hexylthiophene) (P3HT). A detailed description of our experimental set-up and data processing procedure is also given.

引用

页码：1307 / 1319

页数：13

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