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Coal char particle secondary fragmentation in an entrained-flow coal-water slurry gasifier
被引:12
作者:
Guo, Qinghua
[1
]
Zhang, Zhiqing
[1
]
Xue, Zhicun
[1
]
Gong, Yan
[1
]
Yu, Guangsuo
[1
]
Wang, Fuchen
[1
]
机构:
[1] East China Univ Sci & Technol, Shanghai Engn Res Ctr Coal Gasificat, Minist Educ, Key Lab Coal Gasificat & Energy Chem Engn, Shanghai 200237, Peoples R China
基金:
国家重点研发计划;
关键词:
Coal gasification;
Fragmentation;
Coal char;
Particle size distribution;
PULVERIZED COAL;
BEHAVIOR;
ASH;
COMBUSTION;
GASIFICATION;
TEMPERATURE;
CARBON;
REACTIVITY;
MODEL;
D O I:
10.1016/j.joei.2018.04.001
中图分类号:
TE [石油、天然气工业];
TK [能源与动力工程];
学科分类号:
0807 ;
0820 ;
摘要:
Coal char particle size in the gasifier has an influence on the carbon conversion, gasifier slagging as well as the particle matter content in raw syngas. The particle size distribution in a bench-scale opposed multi-burner (OMB) gasifier illustrated that the secondary fragmentation behavior exists in the entrained-flow gasifier after the particles moving from high temperature impinging flame region to the gasification chamber outlet region. Particles larger than 200 mu m in the impinging flame region have porosity structures with fragile shapes. Particle size distributions under different oxygen to carbon ratios (O/C) also indicate that there is an obvious fragmentation while the particle size is larger than 200 mu m. As long as the coal char particles move from the impinging flame region towards the gasification chamber outlet region, the secondary fragmentation is probably taken place as a result of percolative fragmentation, undergoing gasification reactions and thermal stress. However, thermal stress fragmentation only has an influence on the particle sizes larger than 350 mu m according to the calculation by a simplified mathematical model. (C) 2018 Energy Institute. Published by Elsevier Ltd. All rights reserved.
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页码:578 / 586
页数:9
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