Enhancement of the optical properties of CsPbBr3 perovskite nanocrystals using three different solvents

被引:6
作者
Kang, Tae Wook [1 ]
Lee, Sol [1 ]
Park, Young Ji [1 ]
Jeong, Gyu Jin [1 ,2 ]
Kim, Jong Su [3 ]
Bae, Byungseo [4 ]
Hwang, Jonghee [1 ]
Kim, Sun Woog [1 ]
机构
[1] Korea Inst Ceram Engn & Technol, Opt & Elect Component Mat Ctr, Elect Convergence Mat Div, Jinju 52851, South Korea
[2] Gyeongsang Natl Univ, Div Mat Sci & Engn & Convergence Technol, Jinju 52828, South Korea
[3] Pukyong Natl Univ, Dept Display Sci & Engn, Busan 48513, South Korea
[4] Yeongwol Ind Promot Agcy, Adv Resources Team, 21-28 Palgoe 1 Nonggongdanji, Yeongwolgun 26240, South Korea
关键词
CESIUM LEAD HALIDE; LIGHT-EMITTING DEVICES; ANION-EXCHANGE; QUANTUM DOTS; LUMINESCENT; CSPBX3; BR; CL; EMISSION; DIODES;
D O I
10.1364/OL.401058
中图分类号
O43 [光学];
学科分类号
070207 ; 0803 ;
摘要
Green-emitting CsPbBr3 perovskite nanocrystals were synthesized by the modified hot-injection method using three different solvents. The produced nanocrystals showed a narrow green emission band centered at 515-520 nm with full width at half-maximum (FWHM) values of approximately 18-20 nm. The highest photoluminescence quantum yield (PLQY) was obtained for the nanocrystal sample synthesized using a paraffin liquid solvent, with a value of 70.1% under excitation at 450 nm. The CsPbBr3 nanocrystals film light-emitting diodes (LED) chip module showed a luminous efficacy of 40.7 lm/W-rad. The white LED (WLED) with green CsPbBr3 and red CsPbI3 nanocrystal films emitted bluish-white light with a high color rendering index of 89, and the luminous efficacy of the WLED reached 16.31m/W-rad. (C) 2020 Optical Society of America
引用
收藏
页码:4972 / 4975
页数:4
相关论文
共 30 条
[1]   Synthesis of CsPbBr3 and Transformation into Cs4PbBr6 Crystals for White Light Emission with High CRI and Tunable CCT [J].
Adhikari, Gopi C. ;
Thapa, Saroj ;
Zhu, Hongyang ;
Grigoriev, Alexei ;
Zhu, Peifen .
JOURNAL OF PHYSICAL CHEMISTRY C, 2019, 123 (18) :12023-12028
[2]   Saponification Precipitation Method for CsPbBr3 Nanocrystals with Blue-Green Tunable Emission [J].
Adhikari, Gopi C. ;
Vargas, Preston A. ;
Zhu, Hongyang ;
Zhu, Peifen .
JOURNAL OF PHYSICAL CHEMISTRY C, 2019, 123 (02) :1406-1412
[3]   Solution Synthesis Approach to Colloidal Cesium Lead Halide Perovskite Nanoplatelets with Monolayer-Level Thickness Control [J].
Akkerman, Quinten A. ;
Motti, Silvia Genaro ;
Kandada, Ajay Ram Srimath ;
Mosconi, Edoardo ;
D'Innocenzo, Valerio ;
Bertoni, Giovanni ;
Marras, Sergio ;
Kamino, Brett A. ;
Miranda, Laura ;
De Angelis, Filippo ;
Petrozza, Annamaria ;
Prato, Mirko ;
Manna, Liberato .
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY, 2016, 138 (03) :1010-1016
[4]   Tuning the Optical Properties of Cesium Lead Halide Perovskite Nanocrystals by Anion Exchange Reactions [J].
Akkerman, Quinten A. ;
D'Innocenzo, Valerio ;
Accornero, Sara ;
Scarpellini, Alice ;
Petrozza, Annamaria ;
Prato, Mirko ;
Manna, Liberato .
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY, 2015, 137 (32) :10276-10281
[5]   Highly Luminescent Colloidal Nanoplates of Perovskite Cesium Lead Halide and Their Oriented Assemblies [J].
Bekenstein, Yehonadav ;
Koscher, Brent A. ;
Eaton, Samuel W. ;
Yang, Peidong ;
Alivisatos, A. Paul .
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY, 2015, 137 (51) :16008-16011
[6]   Highly Dynamic Ligand Binding and Light Absorption Coefficient of Cesium Lead Bromide Perovskite Nanocrystals [J].
De Roo, Jonathan ;
Ibanez, Maria ;
Geiregat, Pieter ;
Nedelcu, Georgian ;
Walravens, Willem ;
Maes, Jorick ;
Martins, Jose C. ;
Van Driessche, Isabel ;
Koyalenko, Maksym V. ;
Hens, Zeger .
ACS NANO, 2016, 10 (02) :2071-2081
[7]   Room temperature synthesis of stable single silica-coated CsPbBr3 quantum dots combining tunable red emission of Ag-In-Zn-S for High-CRI white light-emitting diodes [J].
Guan, Hongling ;
Zhao, Shuangyi ;
Wang, Huaxin ;
Yan, Dongdong ;
Wang, Ming ;
Zang, Zhigang .
NANO ENERGY, 2020, 67
[8]   Enhanced photoresponse of self-powered perovskite photodetector based on ZnO nanoparticles decorated CsPbBr3 films [J].
Li, Cunlong ;
Han, Ceng ;
Zhang, Yubo ;
Zang, Zhigang ;
Wang, Ming ;
Tang, Xiaosheng ;
Du, Jihe .
SOLAR ENERGY MATERIALS AND SOLAR CELLS, 2017, 172 :341-346
[9]   Highly Efficient Perovskite Nanocrystal Light-Emitting Diodes Enabled by a Universal Crosslinking Method [J].
Li, Guangru ;
Rivarola, Florencia Wisnivesky Rocca ;
Davis, Nathaniel J. L. K. ;
Bai, Sai ;
Jellicoe, Tom C. ;
de la Pena, Francisco ;
Hou, Shaocong ;
Ducati, Caterina ;
Gao, Feng ;
Friend, Richard H. ;
Greenham, Neil C. ;
Tan, Zhi-Kuang .
ADVANCED MATERIALS, 2016, 28 (18) :3528-+
[10]   Healing All-Inorganic Perovskite Films via Recyclable Dissolution-Recyrstallization for Compact and Smooth Carrier Channels of Optoelectronic Devices with High Stability [J].
Li, Xiaoming ;
Yu, Dejian ;
Cao, Fei ;
Gu, Yu ;
Wei, Yi ;
Wu, Ye ;
Song, Jizhong ;
Zeng, Haibo .
ADVANCED FUNCTIONAL MATERIALS, 2016, 26 (32) :5903-5912