Elucidating the origins of the two-dimensional electron gas in LaVO3/SrTiO3 interfaces

被引:3
作者
Hu, L. [1 ]
Wei, R. H. [1 ]
Tang, X. W. [1 ]
Zhu, S. J. [1 ]
Zhang, X. K. [1 ]
Zhu, X. B. [1 ]
Song, W. H. [1 ]
Dai, J. M. [1 ]
Zhang, C. J. [2 ]
Sun, Y. P. [1 ,2 ,3 ]
机构
[1] Chinese Acad Sci, Inst Solid State Phys, Key Lab Mat Phys, Hefei 230031, Anhui, Peoples R China
[2] Chinese Acad Sci, High Magnet Field Lab, Hefei 230031, Anhui, Peoples R China
[3] Collaborat Innovat Ctr Adv Microstruct, Nanjing 210093, Jiangsu, Peoples R China
基金
中国国家自然科学基金; 国家重点研发计划;
关键词
OXIDE INTERFACES; SUPERCONDUCTIVITY; COEXISTENCE; TRANSITION;
D O I
10.1063/1.5085352
中图分类号
O59 [应用物理学];
学科分类号
摘要
The influence of growth rate and substrate temperature on the two-dimensional electron gas (2DEG) of LaVO3/SrTiO3 interfaces has been investigated. It is found that both growth rate and substrate temperature can modulate the structural and electrical properties of the LaVO3/SrTiO3 interfaces through oxygen substrate-to-film transfer. When the LaVO3 thin films are deposited at a low substrate temperature and a high growth rate, the LaVO3/SrTiO3 interfaces exhibit weak oxygen substrate-to-film transfer and resultant low density of oxygen vacancies in the SrTiO3 substrate. As a result, the intrinsic effect (polar discontinuity and/or dielectric screening) dominates the interfacial conduction, while the oxygen vacancies play a minor role. In contrast, the oxygen substrate-to-film transfer (oxygen vacancies in the SrTiO3 substrate) can be enhanced (increased) by depositing the LaVO3 thin films at lower growth rates and/or higher substrate temperatures. In this case, the contribution of oxygen vacancies to the interfacial conduction would prevail over the intrinsic effect. Our results elucidate the origins of 2DEG in the LaVO3/SrTiO3 interfaces and may also be important for other SrTiO3-based heterointerfaces. Published under license by AIP Publishing.
引用
收藏
页数:6
相关论文
共 44 条
[31]   Two components for one resistivity in LaVO3/SrTiO3 heterostructure [J].
Rotella, H. ;
Copie, O. ;
Pautrat, A. ;
Boullay, P. ;
David, A. ;
Pelloquin, D. ;
Labbe, C. ;
Frilay, C. ;
Prellier, W. .
JOURNAL OF PHYSICS-CONDENSED MATTER, 2015, 27 (09)
[32]   Orbital Reconstruction and the Two-Dimensional Electron Gas at the LaAlO3/SrTiO3 Interface [J].
Salluzzo, M. ;
Cezar, J. C. ;
Brookes, N. B. ;
Bisogni, V. ;
De Luca, G. M. ;
Richter, C. ;
Thiel, S. ;
Mannhart, J. ;
Huijben, M. ;
Brinkman, A. ;
Rijnders, G. ;
Ghiringhelli, G. .
PHYSICAL REVIEW LETTERS, 2009, 102 (16)
[33]   The origin of oxygen in oxide thin films: Role of the substrate [J].
Schneider, C. W. ;
Esposito, M. ;
Marozau, I. ;
Conder, K. ;
Doebeli, M. ;
Hu, Yi ;
Mallepell, M. ;
Wokaun, A. ;
Lippert, T. .
APPLIED PHYSICS LETTERS, 2010, 97 (19)
[34]   Oxygen Stoichiometry Effect on Polar Properties of LaAlO3/SrTiO3 [J].
Sharma, Pankaj ;
Huang, Zhen ;
Li, Mengsha ;
Li, Changjian ;
Hu, Songbai ;
Lee, Hyungwoo ;
Lee, Jung-Woo ;
Eom, Chang-Beom ;
Pennycook, Stephen J. ;
Seidel, Jan ;
Ariando ;
Gruverman, Alexei .
ADVANCED FUNCTIONAL MATERIALS, 2018, 28 (23)
[35]   Local resistive switching of Nd doped BiFeO3 thin films [J].
Shen, Wan ;
Bell, Andrew ;
Karimi, Sarah ;
Reaney, Ian M. .
APPLIED PHYSICS LETTERS, 2012, 100 (13)
[36]   High particulate iron(II) content in glacially sourced dusts enhances productivity of a model diatom [J].
Shoenfelt, Elizabeth M. ;
Sun, Jing ;
Winckler, Gisela ;
Kaplan, Michael R. ;
Borunda, Alejandra L. ;
Farrell, Kayla R. ;
Moreno, Patricio I. ;
Gaiero, Diego M. ;
Recasens, Cristina ;
Sambrotto, Raymond N. ;
Bostick, Benjamin C. .
SCIENCE ADVANCES, 2017, 3 (06)
[37]   Observation of inverse Edelstein effect in Rashba-split 2DEG between SrTiO3 and LaAlO3 at room temperature [J].
Song, Qi ;
Zhang, Hongrui ;
Su, Tang ;
Yuan, Wei ;
Chen, Yangyang ;
Xing, Wenyu ;
Shi, Jing ;
Sun, Jirong ;
Han, Wei .
SCIENCE ADVANCES, 2017, 3 (03)
[38]   Two-Dimensional Electron Gases at Complex Oxide Interfaces [J].
Stemmer, Susanne ;
Allen, S. James .
ANNUAL REVIEW OF MATERIALS RESEARCH, VOL 44, 2014, 44 :151-171
[39]   SIMS of thin films grown by pulsed laser deposition on isotopically labeled substrates [J].
Stender, Dieter ;
Cook, Stuart ;
Kilner, John A. ;
Doebeli, Max ;
Conder, Kazimierz ;
Lippert, Thomas ;
Wokaun, Alexander .
SOLID STATE IONICS, 2013, 249 :56-62
[40]   Metal-to-insulator transition in anatase TiO2 thin films induced by growth rate modulation [J].
Tachikawa, T. ;
Minohara, M. ;
Nakanishi, Y. ;
Hikita, Y. ;
Yoshita, M. ;
Akiyama, H. ;
Bell, C. ;
Hwang, H. Y. .
APPLIED PHYSICS LETTERS, 2012, 101 (02)