Elucidating the origins of the two-dimensional electron gas in LaVO3/SrTiO3 interfaces

被引:3
作者
Hu, L. [1 ]
Wei, R. H. [1 ]
Tang, X. W. [1 ]
Zhu, S. J. [1 ]
Zhang, X. K. [1 ]
Zhu, X. B. [1 ]
Song, W. H. [1 ]
Dai, J. M. [1 ]
Zhang, C. J. [2 ]
Sun, Y. P. [1 ,2 ,3 ]
机构
[1] Chinese Acad Sci, Inst Solid State Phys, Key Lab Mat Phys, Hefei 230031, Anhui, Peoples R China
[2] Chinese Acad Sci, High Magnet Field Lab, Hefei 230031, Anhui, Peoples R China
[3] Collaborat Innovat Ctr Adv Microstruct, Nanjing 210093, Jiangsu, Peoples R China
基金
国家重点研发计划; 中国国家自然科学基金;
关键词
OXIDE INTERFACES; SUPERCONDUCTIVITY; COEXISTENCE; TRANSITION;
D O I
10.1063/1.5085352
中图分类号
O59 [应用物理学];
学科分类号
摘要
The influence of growth rate and substrate temperature on the two-dimensional electron gas (2DEG) of LaVO3/SrTiO3 interfaces has been investigated. It is found that both growth rate and substrate temperature can modulate the structural and electrical properties of the LaVO3/SrTiO3 interfaces through oxygen substrate-to-film transfer. When the LaVO3 thin films are deposited at a low substrate temperature and a high growth rate, the LaVO3/SrTiO3 interfaces exhibit weak oxygen substrate-to-film transfer and resultant low density of oxygen vacancies in the SrTiO3 substrate. As a result, the intrinsic effect (polar discontinuity and/or dielectric screening) dominates the interfacial conduction, while the oxygen vacancies play a minor role. In contrast, the oxygen substrate-to-film transfer (oxygen vacancies in the SrTiO3 substrate) can be enhanced (increased) by depositing the LaVO3 thin films at lower growth rates and/or higher substrate temperatures. In this case, the contribution of oxygen vacancies to the interfacial conduction would prevail over the intrinsic effect. Our results elucidate the origins of 2DEG in the LaVO3/SrTiO3 interfaces and may also be important for other SrTiO3-based heterointerfaces. Published under license by AIP Publishing.
引用
收藏
页数:6
相关论文
共 44 条
[1]   VARIATION OF OPTICAL GAPS IN PEROVSKITE-TYPE 3D TRANSITION-METAL OXIDES [J].
ARIMA, T ;
TOKURA, Y ;
TORRANCE, JB .
PHYSICAL REVIEW B, 1993, 48 (23) :17006-17009
[2]   Direct imaging of the coexistence of ferromagnetism and superconductivity at the LaAlO3/SrTiO3 interface [J].
Bert, Julie A. ;
Kalisky, Beena ;
Bell, Christopher ;
Kim, Minu ;
Hikita, Yasuyuki ;
Hwang, Harold Y. ;
Moler, Kathryn A. .
NATURE PHYSICS, 2011, 7 (10) :767-771
[3]   Oxide interfaces for novel electronic applications [J].
Bjaalie, L. ;
Himmetoglu, B. ;
Weston, L. ;
Janotti, A. ;
Van de Walle, C. G. .
NEW JOURNAL OF PHYSICS, 2014, 16
[4]   STRUCTURAL ASPECTS OF THE CRYSTALLOGRAPHIC MAGNETIC TRANSITION IN LAVO3 AROUND 140-K [J].
BORDET, P ;
CHAILLOUT, C ;
MAREZIO, M ;
HUANG, Q ;
SANTORO, A ;
CHEONG, SW ;
TAKAGI, H ;
OGLESBY, CS ;
BATLOGG, B .
JOURNAL OF SOLID STATE CHEMISTRY, 1993, 106 (02) :253-270
[5]   Effect of Growth Induced (Non) Stoichiometry on Interfacial Conductance in LaAlO3/SrTiO3 [J].
Breckenfeld, E. ;
Bronn, N. ;
Karthik, J. ;
Damodaran, A. R. ;
Lee, S. ;
Mason, N. ;
Martin, L. W. .
PHYSICAL REVIEW LETTERS, 2013, 110 (19)
[6]   Magnetic effects at the interface between non-magnetic oxides [J].
Brinkman, A. ;
Huijben, M. ;
Van Zalk, M. ;
Huijben, J. ;
Zeitler, U. ;
Maan, J. C. ;
Van der Wiel, W. G. ;
Rijnders, G. ;
Blank, D. H. A. ;
Hilgenkamp, H. .
NATURE MATERIALS, 2007, 6 (07) :493-496
[7]   Tunable Rashba Spin-Orbit Interaction at Oxide Interfaces [J].
Caviglia, A. D. ;
Gabay, M. ;
Gariglio, S. ;
Reyren, N. ;
Cancellieri, C. ;
Triscone, J. -M. .
PHYSICAL REVIEW LETTERS, 2010, 104 (12)
[8]   High-mobility two-dimensional electron gases at oxide interfaces: Origin and opportunities [J].
Chen Yun-Zhong ;
Pryds, Nini ;
Sun Ji-Rong ;
Shen Bao-Gen ;
Linderoth, Soren .
CHINESE PHYSICS B, 2013, 22 (11)
[9]   Metallic and Insulating Interfaces of Amorphous SrTiO3-Based Oxide Heterostructures [J].
Chen, Yunzhong ;
Pryds, Nini ;
Kleibeuker, Josee E. ;
Koster, Gertjan ;
Sun, Jirong ;
Stamate, Eugen ;
Shen, Baogen ;
Rijnders, Guus ;
Linderoth, Soren .
NANO LETTERS, 2011, 11 (09) :3774-3778
[10]   Structure and magnetism of epitaxial PrVO3 films [J].
Copie, O. ;
Rotella, H. ;
Boullay, P. ;
Morales, M. ;
Pautrat, A. ;
Janolin, P-E ;
Infante, I. C. ;
Pravathana, D. ;
Lueders, U. ;
Prellier, W. .
JOURNAL OF PHYSICS-CONDENSED MATTER, 2013, 25 (49)