Colloidal lead halide perovskite nanocrystals: synthesis, optical properties and applications

被引:408
作者
Huang, He [1 ,2 ]
Polavarapu, Lakshminarayana [3 ,4 ]
Sichert, Jasmina A. [3 ,4 ]
Susha, Andrei S. [1 ,2 ]
Urban, Alexander S. [3 ,4 ]
Rogach, Andrey L. [1 ,2 ]
机构
[1] City Univ Hong Kong, Dept Phys & Mat Sci, 83 Tat Chee Ave, Kowloon Tong, Hong Kong, Peoples R China
[2] City Univ Hong Kong, Ctr Funct Photon, 83 Tat Chee Ave, Kowloon Tong, Hong Kong, Peoples R China
[3] Ludwig Maximilians Univ Munchen, Dept Phys, Amalienstr 54, D-80799 Munich, Germany
[4] Ludwig Maximilians Univ Munchen, CeNS, Amalienstr 54, D-80799 Munich, Germany
关键词
SINGLE-PHOTON EMISSION; SOLAR-CELLS; ROOM-TEMPERATURE; QUANTUM DOTS; ANION-EXCHANGE; SEMICONDUCTOR CLUSTERS; NANOWIRE LASERS; PHASE SYNTHESIS; LUMINESCENT; PHOTOLUMINESCENCE;
D O I
10.1038/am.2016.167
中图分类号
T [工业技术];
学科分类号
08 ;
摘要
Lead halide perovskite nanocrystals (NCs) are receiving a lot of attention nowadays, due to their exceptionally high photoluminescence quantum yields reaching almost 100% and tunability of their optical band gap over the entire visible spectral range by modifying composition or dimensionality/size. We review recent developments in the direct synthesis and ion exchange-based reactions, leading to hybrid organic-inorganic (CH3NH3PbX3) and all-inorganic (CsPbX3) lead halide (X=Cl, Br, I) perovskite NCs, and consider their optical properties related to quantum confinement effects, single emission spectroscopy and lasing. We summarize recent developments on perovskite NCs employed as an active material in several applications such as light-emitting devices, solar cells and photodetectors, and provide a critical outlook into the existing and future challenges.
引用
收藏
页码:e328 / e328
页数:15
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