Revisiting the strategies for stabilizing lithium metal anodes

被引:57
作者
Um, Ji Hyun [1 ]
Kim, Kookhan [2 ,3 ]
Park, Jungjin [4 ]
Sung, Yung-Eun [2 ,3 ]
Yu, Seung-Ho [1 ]
机构
[1] Korea Univ, Dept Chem & Biol Engn, 145 Anam Ro, Seoul 02841, South Korea
[2] Seoul Natl Univ SNU, Sch Chem & Biol Engn, Seoul 08826, South Korea
[3] Inst Basic Sci IBS, Ctr Nanoparticle Res, Seoul 08826, South Korea
[4] Stanford Univ, Dept Mat Sci & Engn, Stanford, CA 94305 USA
基金
新加坡国家研究基金会;
关键词
SOLID-ELECTROLYTE INTERPHASE; POROUS CURRENT COLLECTOR; HIGH IONIC-CONDUCTIVITY; DENDRITE-FREE; POLYMER ELECTROLYTE; IN-SITU; LI-ION; RECHARGEABLE BATTERIES; SUPERCONCENTRATED ELECTROLYTES; NONAQUEOUS ELECTROLYTE;
D O I
10.1039/d0ta03774e
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
The inherent limitations of current lithium-ion batteries for increasing gravimetric and volumetric energy densities with intercalation-based electrode materials have drastically hindered the development of electric vehicles, unmanned aerial vehicles, and stationary energy storage. Lithium metal anodes have been widely considered as promising candidates to overcome the limitations of current anode materials because of their high energy density with low electrochemical potential. However, the unexpected formation of lithium dendrites can cause severe safety concerns and poor coulombic efficiency, which are major obstacles to the commercialization of lithium metal anodes. This review covers the conceptual understanding of current issues and recent advancements in lithium metal battery technologies. In addition, we provide the recommended guidance for commercializing lithium metal batteries.
引用
收藏
页码:13874 / 13895
页数:22
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