Self-assembled CdSe/CdS nanorod micro-lasers fabricated from solution by capillary jet deposition

被引:43
作者
Zavelani-Rossi, Margherita [1 ]
Krahne, Roman [2 ]
Della Valle, Giuseppe [1 ]
Longhi, Stefano [1 ]
Franchini, Isabella R. [3 ]
Girardo, Salvatore [3 ]
Scotognella, Francesco [1 ]
Pisignano, Dario [4 ,5 ]
Manna, Liberato [2 ]
Lanzani, Guglielmo [1 ,6 ]
Tassone, Francesco [6 ]
机构
[1] Politecn Milan, Dipartimento Fis, IFN CNR, I-20133 Milan, Italy
[2] Ist Italiano Tecnol, I-16163 Genoa, Italy
[3] Univ Salento, CNR, Ist Nanosci, NNL, I-73100 Lecce, Italy
[4] Univ Salento, CNR, Dipartimento Matemat & Fis Ennio De Giorgi, NNL,Ist Nanosci, I-73100 Lecce, Italy
[5] IIT UniLe, Ctr Biomol Nanotechnol, I-73010 Lecce, Italy
[6] IIT POLIMI, Ctr Nanosci & Technol, I-20133 Milan, Italy
关键词
ALIGNED SEMICONDUCTOR NANORODS; QUANTUM RODS; OPTICAL GAIN; NANOCRYSTALS;
D O I
10.1002/lpor.201200010
中图分类号
O43 [光学];
学科分类号
070207 ; 0803 ;
摘要
Here we show an innovative, simple and reliable method to fabricate micro-lasers by self-assembly of rod-shaped nanocrystals. We use dot/rod core/shell CdSe/CdS nanorods to form optical micro-resonators by exploiting their self-organization into well-defined coffee stain rings. The fabrication process merely consists of capillary jet deposition of a nanorod solution onto a glass substrate, and is scalable, economic, and highly reproducible. Upon optical pumping of the micro-resonators we obtain laser emission in the red or in the blue-green spectral region, demonstrating lasing both from core and shell transitions, with low pumping thresholds. Modeling by full-wave numerical simulations according to generalized (i. e. scattering) formulation of laser theory demonstrates lasing from complex modes of the self-assembled cavity.
引用
收藏
页码:678 / 683
页数:6
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