Investigating charge-up and fragmentation dynamics of oxygen molecules after interaction with strong X-ray free-electron laser pulses

被引：4

作者：

Kastirke, G. ^{[1
]}

Ota, F. ^{[2
]}

Rezvan, D. V. ^{[3
,4
]}

Schoeffler, M. S. ^{[1
]}

Weller, M. ^{[1
]}

Rist, J. ^{[1
]}

Boll, R. ^{[5
]}

Anders, N. ^{[1
]}

Baumann, T. M. ^{[5
]}

Eckart, S. ^{[1
]}

Erk, B. ^{[6
]}

De Fanis, A. ^{[5
]}

Fehre, K. ^{[1
]}

Gatton, A. ^{[7
]}

Grundmann, S. ^{[1
]}

Grychtol, P. ^{[5
]}

Hartung, A. ^{[1
]}

Hofmann, M. ^{[1
]}

Ilchen, M. ^{[3
,4
,5
]}

Janke, C. ^{[1
]}

Kircher, M. ^{[1
]}

Kunitski, M. ^{[1
]}

Li, X. ^{[8
]}

Mazza, T. ^{[5
]}

Melzer, N. ^{[1
]}

Montano, J. ^{[5
]}

Music, V. ^{[3
,4
,5
]}

Nalin, G. ^{[1
]}

Ovcharenko, Y. ^{[5
]}

Pier, A. ^{[1
]}

Rennhack, N. ^{[5
]}

Rivas, D. E. ^{[5
]}

Doerner, R. ^{[1
]}

Rolles, D. ^{[8
]}

Rudenko, A. ^{[8
]}

Schmidt, Ph. ^{[3
,4
,5
]}

Siebert, J. ^{[1
]}

Strenger, N. ^{[1
]}

Trabert, D. ^{[1
]}

Vela-Perez, I. ^{[1
]}

Wagner, R. ^{[5
]}

Weber, Th. ^{[9
]}

Williams, J. B. ^{[10
]}

Ziolkowski, P. ^{[5
]}

Schmidt, L. Ph. H. ^{[1
]}

Czasch, A. ^{[1
]}

Tamura, Y. ^{[2
]}

Hara, N. ^{[2
]}

Yamazaki, K. ^{[11
]}

Hatada, K. ^{[2
]}

机构：

[1] Goethe Univ, Inst Kernphys, Max Von Laue Str 1, D-60438 Frankfurt, Germany

[2] Univ Toyama, Dept Phys, Gofuku 3190, Toyama 9308555, Japan

[3] Univ Kassel, Inst Phys, Heinrich Plett Str 40, D-34132 Kassel, Germany

[4] Univ Kassel, CINSaT, Heinrich Plett Str 40, D-34132 Kassel, Germany

[5] European XFEL, Holzkoppel 4, D-22869 Schenefeld, Germany

[6] Deutsch Elektronen Synchrotron DESY, Notkestr 85, D-22607 Hamburg, Germany

[7] SLAC Natl Accelerator Lab, Menlo Pk, CA 94025 USA

[8] Kansas State Univ, Dept Phys, JR Macdonald Lab, Manhattan, KS 66506 USA

[9] Lawrence Berkeley Natl Lab, Chem Sci Div, Berkeley, CA 94720 USA

[10] Univ Nevada, Dept Phys, Reno, NV 89557 USA

[11] RIKEN, RIKEN Ctr Adv Photon, 2-1 Hirosawa, Wako, Saitama 3510198, Japan

[12] Fritz Haber Inst Max Planck Gesellschaft, Mol Phys, Faradayweg 4-6, D-14195 Berlin, Germany

[13] Tohoku Univ, Inst Multidisciplinary Res Adv Mat, Katahira 2-1-1,Aoba Ku, Sendai 9808577, Japan

[14] Tohoku Univ, Dept Chem, 6-3 Aramaki Aza Aoba,Aoba Ku, Sendai 9808578, Japan

来源：

PHYSICAL CHEMISTRY CHEMICAL PHYSICS | 2022年 / 24卷 / 44期

基金：

美国国家科学基金会;

关键词：

SPECTROSCOPY; SPACE; ATOMS;

D O I：

10.1039/d2cp02408j

中图分类号：

O64 [物理化学（理论化学）、化学物理学];

学科分类号：

070304 ; 081704 ;

摘要：

During the last decade, X-ray free-electron lasers (XFELs) have enabled the study of light-matter interaction under extreme conditions. Atoms which are subject to XFEL radiation are charged by a complex interplay of (several subsequent) photoionization events and electronic decay processes within a few femtoseconds. The interaction with molecules is even more intriguing, since intricate nuclear dynamics occur as the molecules start to dissociate during the charge-up process. Here, we demonstrate that by analyzing photoelectron angular emission distributions and kinetic energy release of charge states of ionic molecular fragments, we can obtain a detailed understanding of the charge-up and fragmentation dynamics. Our novel approach allows for gathering such information without the need of complex ab initio modeling. As an example, we provide a detailed view on the processes happening on a femtosecond time scale in oxygen molecules exposed to intense XFEL pulses.

引用

页码：27121 / 27127

页数：7

共 40 条

[1] Shape-resonance-enhanced vibrational effects in the angular distributions of C 1s photoelectrons from fixed-in-space CO molecules -: art. no. 163001 [J].

Adachi, J ;

Hosaka, K ;

Furuya, S ;

Soejima, K ;

Takahashi, M ;

Yagishita, A ;

Semenov, SK ;

Cherepkov, NA .

PHYSICAL REVIEW LETTERS, 2003, 91 (16) :163001-163001

[2] Detailed theoretical and experimental description of normal Auger decay in O2 [J].

Bao, Zhuo ;

Fink, Reinhold F. ;

Travnikova, Oksana ;

Ceolin, Denis ;

Svensson, Svante ;

Piancastelli, Maria Novella .

JOURNAL OF PHYSICS B-ATOMIC MOLECULAR AND OPTICAL PHYSICS, 2008, 41 (12)

[3] Double-core-hole spectroscopy for chemical analysis with an intense X-ray femtosecond laser [J].

Berrah, Nora ;

Fang, Li ;

Murphy, Brendan ;

Osipov, Timur ;

Ueda, Kiyoshi ;

Kukk, Edwin ;

Feifel, Raimund ;

van der Meulen, Peter ;

Salen, Peter ;

Schmidt, Henning T. ;

Thomas, Richard D. ;

Larsson, Mats ;

Richter, Robert ;

Prince, Kevin C. ;

Bozek, John D. ;

Bostedt, Christoph ;

Wada, Shin-ichi ;

Piancastelli, Maria N. ;

Tashiro, Motomichi ;

Ehara, Masahiro .

PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA, 2011, 108 (41) :16912-16915

[4] Femtosecond photoelectron diffraction on laser-aligned molecules: Towards time-resolved imaging of molecular structure [J].

Boll, R. ;

Anielski, D. ;

Bostedt, C. ;

Bozek, J. D. ;

Christensen, L. ;

Coffee, R. ;

De, S. ;

Decleva, P. ;

Epp, S. W. ;

Erk, B. ;

Foucar, L. ;

Krasniqi, F. ;

Kuepper, J. ;

Rouzee, A. ;

Rudek, B. ;

Rudenko, A. ;

Schorb, S. ;

Stapelfeldt, H. ;

Stener, M. ;

Stern, S. ;

Techert, S. ;

Trippel, S. ;

Vrakking, M. J. J. ;

Ullrich, J. ;

Rolles, D. .

PHYSICAL REVIEW A, 2013, 88 (06)

[5] Conformer-specific photochemistry imaged in real space and time [J].

Champenois, E. G. ;

Sanchez, D. M. ;

Yang, J. ;

Nunes, J. P. Figueira ;

Attar, A. ;

Centurion, M. ;

Forbes, R. ;

Guhr, M. ;

Hegazy, K. ;

Ji, F. ;

Saha, S. K. ;

Liu, Y. ;

Lin, M-F ;

Luo, D. ;

Moore, B. ;

Shen, X. ;

Ware, M. R. ;

Wang, X. J. ;

Martinez, T. J. ;

Wolf, T. J. A. .

SCIENCE, 2021, 374 (6564) :178-182

[6] Femtosecond X-ray protein nanocrystallography [J].

Chapman, Henry N. ;

Fromme, Petra ;

Barty, Anton ;

White, Thomas A. ;

Kirian, Richard A. ;

Aquila, Andrew ;

Hunter, Mark S. ;

Schulz, Joachim ;

DePonte, Daniel P. ;

Weierstall, Uwe ;

Doak, R. Bruce ;

Maia, Filipe R. N. C. ;

Martin, Andrew V. ;

Schlichting, Ilme ;

Lomb, Lukas ;

Coppola, Nicola ;

Shoeman, Robert L. ;

Epp, Sascha W. ;

Hartmann, Robert ;

Rolles, Daniel ;

Rudenko, Artem ;

Foucar, Lutz ;

Kimmel, Nils ;

Weidenspointner, Georg ;

Holl, Peter ;

Liang, Mengning ;

Barthelmess, Miriam ;

Caleman, Carl ;

Boutet, Sebastien ;

Bogan, Michael J. ;

Krzywinski, Jacek ;

Bostedt, Christoph ;

Bajt, Sasa ;

Gumprecht, Lars ;

Rudek, Benedikt ;

Erk, Benjamin ;

Schmidt, Carlo ;

Hoemke, Andre ;

Reich, Christian ;

Pietschner, Daniel ;

Strueder, Lothar ;

Hauser, Guenter ;

Gorke, Hubert ;

Ullrich, Joachim ;

Herrmann, Sven ;

Schaller, Gerhard ;

Schopper, Florian ;

Soltau, Heike ;

Kuehnel, Kai-Uwe ;

Messerschmidt, Marc .

NATURE, 2011, 470 (7332) :73-U81

[7] Single center method: A computational tool for ionization and electronic excitation studies of molecules [J].

Demekhin, Ph V. ;

Ehresmann, A. ;

Sukhorukov, V. L. .

JOURNAL OF CHEMICAL PHYSICS, 2011, 134 (02)

[8] CALCULATING PROPERTIES WITH THE COHERENT-POTENTIAL APPROXIMATION [J].

FAULKNER, JS ;

STOCKS, GM .

PHYSICAL REVIEW B, 1980, 21 (08) :3222-3244

[9] Probing molecular bond-length using molecular-frame photoelectron angular distributions [J].

Fukuzawa, Hironobu ;

Lucchese, Robert R. ;

Liu, Xiao-Jing ;

Sakai, Kentaro ;

Iwayama, Hiroshi ;

Nagaya, Kiyonobu ;

Kreidi, Katharina ;

Schoeffler, Markus S. ;

Harries, James R. ;

Tamenori, Yusuke ;

Morishita, Yuichiro ;

Suzuki, Isao H. ;

Saito, Norio ;

Ueda, Kiyoshi .

JOURNAL OF CHEMICAL PHYSICS, 2019, 150 (17)

[10] Hartree-Fock calculation of the differential photoionization cross sections of small Li clusters [J].

Galitskiy, S. A. ;

Artemyev, A. N. ;

Jankala, K. ;

Lagutin, B. M. ;

Demekhin, Ph. V. .

JOURNAL OF CHEMICAL PHYSICS, 2015, 142 (03)

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