Highly Luminescent and Stable Halide Perovskite Nanocrystals

被引:151
作者
Wu, Ye [1 ]
Li, Xiaoming [1 ]
Zeng, Haibo [1 ]
机构
[1] Nanjing Univ Sci & Technol, Inst Optoelect & Nanomat, Coll Mat Sci & Engn, MIIT Key Lab Adv Display Mat & Devices, Nanjing 210094, Jiangsu, Peoples R China
来源
ACS ENERGY LETTERS | 2019年 / 4卷 / 03期
基金
国家杰出青年科学基金;
关键词
LIGHT-EMITTING-DIODES; EXTERNAL QUANTUM EFFICIENCY; BLUE; SEGREGATION; DOTS; STRATEGY; CSPBX3; GREEN; CL; BR;
D O I
10.1021/acsenergylett.8b02100
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
Lead halide perovskites are potential candidates for wide-color-gamut display applications. Recently, red and green light-emitting diodes (LEDs) based on these materials have achieved external quantum efficiency (EQE) of over 20%, while the blue devices lag behind them severely because of a much lower photoluminescence quantum yield (PL QY) and inferior stability. Blue perovskite nanocrystals (NCs) are promising active materials for high-efficiency devices; however, they are reported to exhibit low defect tolerance and suffer from troublesome ion migration behavior. Though some good ideas have been proposed to overcome these problems, the present results are still unsatisfactory. In this Perspective, diverse methods toward blue perovskite NCs are summarized, as well as the intrinsic origin of low stability and poor optical properties. Then, strategies to improve their performance and stability and critical challenges that severely limit the stability and performances of blue perovskite NCs are discussed. Perspectives of further developments on synthesis and applications of blue perovskite NCs are both provided.
引用
收藏
页码:673 / 681
页数:17
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