Graphitic C3N4-Sensitized TiO2 Nanotube Layers: A Visible-Light Activated Efficient Metal-Free Antimicrobial Platform

被引：64

作者：

Xu, Jingwen ^{[1
]}

Li, Yan ^{[1
]}

Zhou, Xuemei ^{[2
]}

Li, Yuzhen ^{[1
]}

Gao, Zhi-Da ^{[1
]}

Song, Yan-Yan ^{[1
]}

Schmuki, Patrik ^{[2
,3
]}

机构：

[1] Northeastern Univ, Coll Sci, Box 332, Shenyang 110004, Peoples R China

[2] WW4 LKO Univ Erlangen Nuremberg, Dept Mat Sci, Martensstr 7, D-91058 Erlangen, Germany

[3] King Abdulaziz Univ, Fac Sci, Dept Chem, POB 80203, Jeddah 21569, Saudi Arabia

来源：

CHEMISTRY-A EUROPEAN JOURNAL | 2016年 / 22卷 / 12期

基金：

中国国家自然科学基金;

关键词：

antibacterial agents; C3N4; TiO2; nanotubes; vapor deposition; visible-light; CARBON NITRIDE; PHOTOCATALYST; SURFACES; GRAPHENE; ARRAYS;

D O I：

10.1002/chem.201505173

中图分类号：

O6 [化学];

学科分类号：

0703 ;

摘要：

Herein, we use a facile procedure to graft a thin graphitic C3N4 (g-C3N4) layer on aligned TiO2 nanotube arrays (TiNT) by a one-step chemical vapor deposition (CVD) approach. This provides a platform to enhance the visible-light response of TiO2 nanotubes for antimicrobial applications. The formed g-C3N4/TiNT binary nanocomposite exhibits excellent bactericidal efficiency against Escherichia coli (E. coli) as a visible-light activated antibacterial coating, without the use of additional bactericides.

引用

页码：3947 / 3951

页数：5

共 33 条

[1] One pot synthesis and characterization of Ag-ZnO/g-C3N4 photocatalyst with improved photoactivity and antibacterial properties [J].

Adhikari, Surya Prasad ;

Pant, Hem Raj ;

Kim, Jun Hee ;

Kim, Han Joo ;

Park, Chan Hee ;

Kim, Cheol Sang .

COLLOIDS AND SURFACES A-PHYSICOCHEMICAL AND ENGINEERING ASPECTS, 2015, 482 :477-484

[2]

[Anonymous], 2006, ANGEW CHEM INT EDIT

[3] Visible-light photocatalysis in nitrogen-doped titanium oxides [J].

Asahi, R ;

Morikawa, T ;

Ohwaki, T ;

Aoki, K ;

Taga, Y .

SCIENCE, 2001, 293 (5528) :269-271

[4] Epidemiology of methicillin-resistant Staphylococcus aureus [J].

Boucher, Helen W. ;

Corey, G. Ralph .

CLINICAL INFECTIOUS DISEASES, 2008, 46 :S344-S349

[5] Bacterial biofilms: A common cause of persistent infections [J].

Costerton, JW ;

Stewart, PS ;

Greenberg, EP .

SCIENCE, 1999, 284 (5418) :1318-1322

[6] Efficacy of antiadhesive, antibiotic and antiseptic coatings in preventing catheter-related infections: Review [J].

Donelli, G ;

Francolini, I .

JOURNAL OF CHEMOTHERAPY, 2001, 13 (06) :595-606

[7] ELECTROCHEMICAL PHOTOLYSIS OF WATER AT A SEMICONDUCTOR ELECTRODE [J].

FUJISHIMA, A ;

HONDA, K .

NATURE, 1972, 238 (5358) :37-+

[8] Chemical synthesis of mesoporous carbon nitrides using hard templates and their use as a metal-free catalyst for friedel-crafts reaction of benzene [J].

Goettmann, Frederic ;

Fischer, Anna ;

Antonietti, Markus ;

Thomas, Arne .

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION, 2006, 45 (27) :4467-4471

[9] Properties of O2•- and OH• formed in TiO2 aqueous suspensions by photocatalytic reaction and the influence of H2O2 and some ions [J].

Hirakawa, T ;

Nosaka, Y .

LANGMUIR, 2002, 18 (08) :3247-3254

[10] ENVIRONMENTAL APPLICATIONS OF SEMICONDUCTOR PHOTOCATALYSIS [J].

HOFFMANN, MR ;

MARTIN, ST ;

CHOI, WY ;

BAHNEMANN, DW .

CHEMICAL REVIEWS, 1995, 95 (01) :69-96

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