Removing cross-phase modulation from midinfrared chirped-pulse upconversion spectra

被引:31
|
作者
Lee, Kevin F. [1 ]
Nuernberger, Patrick
Bonvalet, Adeline
Joffre, Manuel
机构
[1] Ecole Polytech, CNRS, Lab Opt & Biosci, F-91128 Palaiseau, France
来源
OPTICS EXPRESS | 2009年 / 17卷 / 21期
关键词
2-DIMENSIONAL INFRARED-SPECTROSCOPY; ELECTRIC-FIELD RECONSTRUCTION; SHAPED ULTRAVIOLET PULSES; SUM-FREQUENCY GENERATION; LASER-PULSES; INTERFEROMETRY; SPECTROMETER; RESOLUTION;
D O I
10.1364/OE.17.018738
中图分类号
O43 [光学];
学科分类号
070207 ; 0803 ;
摘要
We observe that narrow spectral features in mid-infrared spectra obtained by chirped-pulse up-conversion are strongly distorted by cross-phase modulation between the mid-infrared field and the chirped pulse. We discuss the consequences of this effect on spectral resolution, and introduce a correction method that recovers masked lines. This simple correction can be applied either when the upconverted field is fully characterized, such as in multidimensional spectroscopy, or when causality can be used, such as in absorption spectroscopy, which we demonstrate experimentally. (C) 2009 Optical Society of America
引用
收藏
页码:18738 / 18744
页数:7
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