Impedance measurements on QLED devices: analysis of high-frequency loop in terms of material properties

被引:8
作者
You, Chen [1 ]
Titov, Alex [2 ]
Kim, Baek Hyun [2 ]
Orazem, Mark E. [1 ]
机构
[1] Univ Florida, Dept Chem Engn, Gainesville, FL 32611 USA
[2] NanoPhotonica Inc, Res Lab, UF Innovate Hub, Gainesville, FL 32601 USA
关键词
Quantum-dot light-emitting diodes; Electrochemical impedance spectroscopy; Power-law model; Regression analysis; LIGHT-EMITTING-DIODES; MEASUREMENT MODELS; RESISTIVITY DISTRIBUTIONS; SPECTROSCOPY;
D O I
10.1007/s10008-020-04765-1
中图分类号
O646 [电化学、电解、磁化学];
学科分类号
081704 ;
摘要
Electrochemical impedance spectroscopy is used to study red and green quantum-dot light-emitting diodes devices. The high-frequency loop is interpreted in terms of the thickness, dielectric constant, and resistivity distribution of the hole-injection layer. The analysis employed the device capacitance obtained from a measurement model analysis, the film thickness measured by scanning electron microscopy, and an interpretation of the impedance based on a power-law model. Impedance measurements performed on hole-transport-only devices yielded results that were consistent with the interpretation of the high-frequency capacitive loop in terms of the properties of the hole-injection layer.
引用
收藏
页码:3083 / 3090
页数:8
相关论文
共 19 条
  • [1] MEASUREMENT MODELS FOR ELECTROCHEMICAL IMPEDANCE SPECTROSCOPY .1. DEMONSTRATION OF APPLICABILITY
    AGARWAL, P
    ORAZEM, ME
    GARCIARUBIO, LH
    [J]. JOURNAL OF THE ELECTROCHEMICAL SOCIETY, 1992, 139 (07) : 1917 - 1927
  • [2] Application of measurement models to impedance spectroscopy .2. Determination of the stochastic contribution to the error structure
    Agarwal, P
    Crisalle, OD
    Orazem, ME
    GarciaRubio, LH
    [J]. JOURNAL OF THE ELECTROCHEMICAL SOCIETY, 1995, 142 (12) : 4149 - 4158
  • [3] Application of measurement models to impedance spectroscopy .3. Evaluation of consistency with the Kramers-Kronig relations
    Agarwal, P
    Orazem, ME
    GarciaRubio, LH
    [J]. JOURNAL OF THE ELECTROCHEMICAL SOCIETY, 1995, 142 (12) : 4159 - 4168
  • [4] Constant-phase-element behavior caused by inhomogeneous water uptake in anti-corrosion coatings
    Amand, Sylvain
    Musiani, Marco
    Orazem, Mark E.
    Pebere, Nadine
    Tribollet, Bernard
    Vivier, Vincent
    [J]. ELECTROCHIMICA ACTA, 2013, 87 : 693 - 700
  • [5] [Anonymous], 2017, Tribollet Electrochemical Impedance Spectroscopy, DOI DOI 10.1002/9781119363682
  • [6] Study of Hole-Injecting Properties in Efficient, Stable, and Simplified Phosphorescent Organic Light-Emitting Diodes by Impedance Spectroscopy
    Cai, S. D.
    Gao, C. H.
    Zhou, D. Y.
    Gu, W.
    Liao, L. S.
    [J]. ACS APPLIED MATERIALS & INTERFACES, 2012, 4 (01) : 312 - 316
  • [7] Impedance spectroscopy of OLEDs as a tool for estimating mobility and the concentration of charge carriers in transport layers
    Chulkin, P.
    Vybornyi, O.
    Lapkowski, M.
    Skabara, P. J.
    Data, P.
    [J]. JOURNAL OF MATERIALS CHEMISTRY C, 2018, 6 (05) : 1008 - 1014
  • [8] Determination of standard redox rate constants of OLED active compounds by electrochemical impedance spectroscopy
    Chulkin, Pavel
    Lapkowski, Mieczyslaw
    Bryce, Martin R.
    Santos, Jose
    Data, Przemyslaw
    [J]. ELECTROCHIMICA ACTA, 2017, 258 : 1160 - 1172
  • [9] Hirschorn B, 2010, J ELECTROCHEM SOC, V157, pC458, DOI 10.1149/1.3499565
  • [10] Constant-Phase-Element Behavior Caused by Resistivity Distributions in Films I. Theory
    Hirschorn, Bryan
    Orazem, Mark E.
    Tribollet, Bernard
    Vivier, Vincent
    Frateur, Isabelle
    Musiani, Marco
    [J]. JOURNAL OF THE ELECTROCHEMICAL SOCIETY, 2010, 157 (12) : C452 - C457