Generation of ultrafast terahertz radiation pulses on metallic nanostructured surfaces

被引:88
作者
Welsh, Gregor H. [1 ]
Wynne, Klaas [1 ]
机构
[1] Univ Strathclyde, Dept Phys, SUPA, Glasgow G4 0NG, Lanark, Scotland
基金
英国工程与自然科学研究理事会;
关键词
EVANESCENT-WAVE ACCELERATION; OPTICAL RECTIFICATION; CHARGE-TRANSFER; EMISSION; FILMS; FIELD; PHOTOEMISSION; SPECTROSCOPY; MULTIPHOTON; EXCITATION;
D O I
10.1364/OE.17.002470
中图分类号
O43 [光学];
学科分类号
070207 ; 0803 ;
摘要
A resonant "incoherent" rectification process is presented relying on the excitation of surface plasmons on a nanostructured metal surface. Excitation of gold and silver films with 800-nm femtosecond laser pulses results in the emission of terahertz radiation with an angle-dependent efficiency and an approximately third-order power dependence. It is shown that the source of this terahertz pulse generation is the surface-plasmon-assisted multiphoton ionization and ponderomotive acceleration in the evanescent field of the surface plasmon. Simple models are used to understand the forces and dynamics near the surface. (C) 2009 Optical Society of America
引用
收藏
页码:2470 / 2480
页数:11
相关论文
共 39 条
[1]   OBSERVATION OF SURFACE-ENHANCED MULTIPHOTON PHOTOEMISSION FROM METAL-SURFACES IN THE SHORT-PULSE LIMIT [J].
AESCHLIMANN, M ;
SCHMUTTENMAER, CA ;
ELSAYEDALI, HE ;
MILLER, RJD ;
CAO, J ;
GAO, Y ;
MANTELL, DA .
JOURNAL OF CHEMICAL PHYSICS, 1995, 102 (21) :8606-8613
[2]   PICOSECOND PHOTOCONDUCTING HERTZIAN DIPOLES [J].
AUSTON, DH ;
CHEUNG, KP ;
SMITH, PR .
APPLIED PHYSICS LETTERS, 1984, 45 (03) :284-286
[3]   Enhanced electronic emission by excitation of an interface resonance in metallic bilayer gratings irradiated by short laser pulses [J].
Bastiani-Ceccotti, S ;
Monchicourt, P ;
Lehner, T .
PHYSICAL REVIEW B, 2003, 68 (24)
[4]  
Beard MC, 2002, J PHYS CHEM A, V106, P878, DOI [10.1021/jp013603l, 10.1021/jp0136031]
[5]   Coherent terahertz emission from ferromagnetic films excited by femtosecond laser pulses [J].
Beaurepaire, E ;
Turner, GM ;
Harrel, SM ;
Beard, MC ;
Bigot, JY ;
Schmuttenmaer, CA .
APPLIED PHYSICS LETTERS, 2004, 84 (18) :3465-3467
[6]   Terahertz pulse generation in an organic crystal by optical rectification and resonant excitation of molecular charge transfer [J].
Carey, JJ ;
Bailey, RT ;
Pugh, D ;
Sherwood, JN ;
Cruickshank, FR ;
Wynne, K .
APPLIED PHYSICS LETTERS, 2002, 81 (23) :4335-4337
[7]   Corrosion at the nanoscale: The case of silver nanowires and nanoparticles [J].
Elechiguerra, JL ;
Larios-Lopez, L ;
Liu, C ;
Garcia-Gutierrez, D ;
Camacho-Bragado, A ;
Yacaman, MJ .
CHEMISTRY OF MATERIALS, 2005, 17 (24) :6042-6052
[8]   INTENSE SURFACE PHOTOEMISSION - SPACE-CHARGE EFFECTS AND SELF-ACCELERATION [J].
GILTON, TL ;
COWIN, JP ;
KUBIAK, GD ;
HAMZA, AV .
JOURNAL OF APPLIED PHYSICS, 1990, 68 (09) :4802-4810
[9]   FIELD-EMISSION, FIELD-IONIZATION, AND FIELD DESORPTION [J].
GOMER, R .
SURFACE SCIENCE, 1994, 299 (1-3) :129-152
[10]   FAR-INFRARED TIME-DOMAIN SPECTROSCOPY WITH TERAHERTZ BEAMS OF DIELECTRICS AND SEMICONDUCTORS [J].
GRISCHKOWSKY, D ;
KEIDING, S ;
VANEXTER, M ;
FATTINGER, C .
JOURNAL OF THE OPTICAL SOCIETY OF AMERICA B-OPTICAL PHYSICS, 1990, 7 (10) :2006-2015