Near-Field Plasmonics of an Individual Dielectric Nanoparticle above a Metallic Substrate

被引:58
作者
Hutter, Tanya [1 ]
Huang, Fu Min [2 ]
Elliott, Stephen R. [1 ]
Mahajan, Sumeet [2 ,3 ]
机构
[1] Univ Cambridge, Dept Chem, Cambridge CB2 1EW, England
[2] Univ Cambridge, Cavendish Lab, Dept Phys, Cambridge CB3 0HE, England
[3] Univ Southampton, Inst Life Sci, Southampton SO17 1BJ, Hants, England
基金
英国工程与自然科学研究理事会;
关键词
ENHANCED RAMAN-SCATTERING; RESONANCE;
D O I
10.1021/jp400963f
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
We simulate and discuss the local electric-field enhancement in a system of a dielectric nanoparticle placed very near to a metallic substrate. We use finite-element numerical simulations in order to understand the field-enhancement mechanism in this dielectric NP-on-mirror system. Under appropriate excitation conditions, the gap between the particle and the substrate becomes a "hot spot", i.e., a region of intense electromagnetic field. We also show how the optical properties of the dielectric NP placed on a metallic substrate affect the plasmonic field enhancement in the nanogap and characterize the confinement in the gap. Our study helps to understand and design systems with dielectric NPs on metallic substrates which can be equally as effective for SERS, fluorescence, and nonlinear phenomena as conventional all plasmonic structures.
引用
收藏
页码:7784 / 7790
页数:7
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