MoS2-reduced graphene oxide composites synthesized via a microwave-assisted method for visible-light photocatalytic degradation of methylene blue

被引:123
作者
Li, Jinliang [1 ]
Liu, Xinjuan [2 ]
Pan, Likun [1 ]
Qin, Wei [1 ]
Chen, Taiqiang [1 ]
Sun, Zhuo [1 ]
机构
[1] E China Normal Univ, Dept Phys, Engn Res Ctr Nanophoton & Adv Instrument, Minist Educ,Shanghai Key Lab Magnet Resonance, Shanghai 200062, Peoples R China
[2] Shanghai Nanotechnol Promot Ctr, Shanghai 200237, Peoples R China
基金
中国博士后科学基金;
关键词
HYDROGEN EVOLUTION; TIO2-GRAPHENE NANOCOMPOSITES; ENHANCED PHOTOCATALYSIS; HIGH-PERFORMANCE; LAYER MOS2; ZNO; NANOPARTICLES; TIO2; DYES; REDUCTION;
D O I
10.1039/c3ra46956e
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
MoS2-reduced graphene oxide (RGO) composites were successfully synthesized via microwave-assisted reduction of graphite oxide in a MoS2 precursor aqueous solution using a microwave system. The morphology, structure and photocatalytic performance in the degradation of methylene blue (MB) were characterized by scanning electron microscopy, X-ray diffraction, electrochemical impedance spectra and UV-vis absorption spectroscopy, respectively. The results show that the MoS2-RGO composites exhibit enhanced photocatalytic performance in the degradation of MB with a maximum degradation rate of 99% under visible light irradiation for 60 min. This excellent photocatalytic activity is due to the contribution from the reduced electron-hole pair recombination, the enhanced light absorption and the increased dye adsorptivity with the introduction of RGO in the composite.
引用
收藏
页码:9647 / 9651
页数:5
相关论文
共 55 条
[1]   WO3 nanorods/graphene nanocomposites for high-efficiency visible-light-driven photocatalysis and NO2 gas sensing [J].
An, Xiaoqiang ;
Yu, Jimmy C. ;
Wang, Yu ;
Hu, Yongming ;
Yu, Xuelian ;
Zhang, Guangjin .
JOURNAL OF MATERIALS CHEMISTRY, 2012, 22 (17) :8525-8531
[2]   Performance Enhancement of ZnO Photocatalyst via Synergic Effect of Surface Oxygen Defect and Graphene Hybridization [J].
Bai, Xiaojuan ;
Wang, Li ;
Zong, Ruilong ;
Lv, Yanhui ;
Sun, Yiqing ;
Zhu, Yongfa .
LANGMUIR, 2013, 29 (09) :3097-3105
[3]   Ripples and Layers in Ultrathin MoS2 Membranes [J].
Brivio, Jacopo ;
Alexander, Duncan T. L. ;
Kis, Andras .
NANO LETTERS, 2011, 11 (12) :5148-5153
[4]   In situ synthesis of MoS2/graphene nanosheet composites with extraordinarily high electrochemical performance for lithium ion batteries [J].
Chang, Kun ;
Chen, Weixiang .
CHEMICAL COMMUNICATIONS, 2011, 47 (14) :4252-4254
[5]   Reduction degree of reduced graphene oxide (RGO) dependence of photocatalytic hydrogen evolution performance over RGO/ZnIn2S4 nanocomposites [J].
Chen, Yongjuan ;
Ge, Hao ;
Wei, Liang ;
Li, Zhaohui ;
Yuan, Rusheng ;
Liu, Ping ;
Fu, Xianzhi .
CATALYSIS SCIENCE & TECHNOLOGY, 2013, 3 (07) :1712-1717
[6]   Photoluminescence from Chemically Exfoliated MoS2 [J].
Eda, Goki ;
Yamaguchi, Hisato ;
Voiry, Damien ;
Fujita, Takeshi ;
Chen, Mingwei ;
Chhowalla, Manish .
NANO LETTERS, 2011, 11 (12) :5111-5116
[7]   CdSe-MoS2: A Quantum Size-Confined Photocatalyst for Hydrogen Evolution from Water under Visible Light [J].
Frame, F. Andrew ;
Osterloh, Frank E. .
JOURNAL OF PHYSICAL CHEMISTRY C, 2010, 114 (23) :10628-10633
[8]   Combination of cobalt ferrite and graphene: High-performance and recyclable visible-light photocatalysis [J].
Fu, Yongsheng ;
Chen, Haiqun ;
Sun, Xiaoqiang ;
Wang, Xin .
APPLIED CATALYSIS B-ENVIRONMENTAL, 2012, 111 :280-287
[9]   Selective dehydrogenation of aromatic alcohols photocatalyzed by Pd-deposited CdS-TiO2 in aqueous solution using visible light [J].
Higashimoto, Shinya ;
Tanaka, Yoshimi ;
Ishikawa, Ryo ;
Hasegawa, Shoko ;
Azuma, Masashi ;
Ohue, Hiroyoshi ;
Sakata, Yoshihisa .
CATALYSIS SCIENCE & TECHNOLOGY, 2013, 3 (02) :400-403
[10]   Synthesis and photocatalytic properties of nano-MoS2/kaolin composite [J].
Hu, Kun Hong ;
Liu, Zhu ;
Huang, Fei ;
Hu, Xian Guo ;
Han, Cheng Liang .
CHEMICAL ENGINEERING JOURNAL, 2010, 162 (02) :836-843