Theoretical treatments of radiationless transitions

被引：8

作者：

Chin, CH

Shiu, HYJ

Wang, HW

Chen, YL

Wang, CC

Lin, SH

Hayashi, M ^{[1
]}

机构：

[1] Natl Taiwan Univ, Ctr Condensed Matter Sci, Taipei 10764, Taiwan

[2] Acad Sinica, Inst Atom & Mol Sci, Taipei 10764, Taiwan

来源：

JOURNAL OF THE CHINESE CHEMICAL SOCIETY | 2006年 / 53卷 / 01期

关键词：

photo-induced; radiationless transition; non-adiabatic processes; vibronic theory; rate constants;

D O I：

10.1002/jccs.200600016

中图分类号：

O6 [化学];

学科分类号：

0703 ;

摘要：

In this review, we present a microscopic theory for describing photo-induced radiationless transitions. For this purpose, we state that introducing the density matrix method can not only treat the dynamics due to the radiationless transitions but also deal with the population and coherence dynamics. We briefly review several rate constants of the radiationless transitions and the analytic estimation methods of those rate constants. Finally, we present the applications of the theoretical treatment to the rapid electron transfer and energy transfer taking place in the photosynthetic reaction centers.

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页码：131 / 152

页数：22

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