Charge asymmetric dissociation of a CO+ molecular-ion beam induced by strong laser fields

被引:13
|
作者
Kling, Nora G. [1 ]
McKenna, J. [1 ]
Sayler, A. M. [1 ]
Gaire, B. [1 ]
Zohrabi, M. [1 ]
Ablikim, U. [1 ]
Carnes, K. D. [1 ]
Ben-Itzhak, I. [1 ]
机构
[1] Kansas State Univ, Dept Phys, JR Macdonald Lab, Manhattan, KS 66506 USA
来源
PHYSICAL REVIEW A | 2013年 / 87卷 / 01期
关键词
DIATOMIC-MOLECULES; POTENTIAL-ENERGY; IONIZATION; FRAGMENTATION; TRANSITION; DYNAMICS; CURVES; BOND;
D O I
10.1103/PhysRevA.87.013418
中图分类号
O43 [光学];
学科分类号
070207 ; 0803 ;
摘要
Charge asymmetric dissociation into C2+ + O following ionization of a CO+ molecular-ion beam with intense ultrashort (7-40-fs) laser pulses is studied using a coincidence three-dimensional momentum imaging method. The data suggest that allowing the molecule enough time to stretch within a laser pulse such that it ionizes beyond the curve crossings of the C2+ + O and C+ + O+ potentials enhances the otherwise hard-to-reach charge asymmetric dissociation channel. DOI: 10.1103/PhysRevA.87.013418
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页数:7
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