Recovery of Uranium from Seawater: A Review of Current Status and Future Research Needs

被引:433
作者
Kim, Jungseung [1 ]
Tsouris, Costas [1 ]
Mayes, Richard T. [1 ]
Oyola, Yatsandra [1 ]
Saito, Tomonori [1 ]
Janke, Christopher J. [1 ]
Dai, Sheng [1 ]
Schneider, Erich [2 ]
Sachde, Darshan [2 ]
机构
[1] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA
[2] Univ Texas Austin, Nucl & Radiat Engn Program, Austin, TX 78712 USA
关键词
uranium adsorbents; uranium adsorption; uranium from seawater; MACRORETICULAR CHELATING RESIN; AMIDOXIME-FIBER ADSORBENTS; HYDROUS METAL-OXIDE; INDUCED GRAFT-COPOLYMERIZATION; MESOPOROUS CARBON MATERIALS; SOLID-PHASE EXTRACTION; SEA-WATER; ACTIVATED CARBON; URANYL IONS; ADSORPTION PROPERTIES;
D O I
10.1080/01496395.2012.712599
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
The recovery of uranium (U) from seawater has been investigated for over six decades in efforts to secure uranium sources for future energy production. The majority of the research activities have focused on inorganic materials, chelating polymers, and nanomaterials. Previous studies of uranium adsorption from aqueous solutions, mainly seawater, are reviewed here with a focus on various adsorbent materials, adsorption parameters, adsorption characterization, and marine studies. Continuous progress has been made over several decades, with adsorbent loadings approaching 3.2 mg U/g adsorbent in equilibrium with seawater. Further research is needed to improve first, the viability including improved capacity, selectivity, and kinetics, and second, the sorbent regeneration for multicycle use. An overview of the status of the uranium adsorption technology is provided and future research needs to make this technology commercially competitive are discussed.
引用
收藏
页码:367 / 387
页数:21
相关论文
共 232 条
[41]   PREPARATION OF MACRORETICULAR CHELATING RESINS CONTAINING DIHYDROXYPHOSPHINO AND OR PHOSPHONO GROUPS AND THEIR ADSORPTION ABILITY FOR URANIUM [J].
EGAWA, H ;
NONAKA, T ;
IKARI, M .
JOURNAL OF APPLIED POLYMER SCIENCE, 1984, 29 (06) :2045-2055
[42]   RECOVERY OF URANIUM FROM SEAWATER .15. DEVELOPMENT OF AMIDOXIME RESINS WITH HIGH SEDIMENTATION-VELOCITY FOR PASSIVELY DRIVER FLUIDIZED-BED ADSORBERS [J].
EGAWA, H ;
KABAY, N ;
JYO, A ;
HIRONO, M ;
SHUTO, T .
INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH, 1994, 33 (03) :657-661
[43]   RECOVERY OF URANIUM FROM SEA-WATER .4. INFLUENCE OF CROSS-LINKING REAGENT ON THE URANIUM ADSORPTION OF MACRORETICULAR CHELATING RESIN CONTAINING AMIDOXIME GROUPS [J].
EGAWA, H ;
NAKAYAMA, M ;
NONAKA, T ;
SUGIHARA, E .
JOURNAL OF APPLIED POLYMER SCIENCE, 1987, 33 (06) :1993-2005
[44]   RECOVERY OF URANIUM FROM SEAWATER .14. SYSTEM ARRANGEMENTS FOR THE RECOVERY OF URANIUM FROM SEAWATER BY SPHERICAL AMIDOXIME CHELATING RESINS UTILIZING NATURAL SEAWATER MOTIONS [J].
EGAWA, H ;
KABAY, N ;
SHUTO, T ;
JYO, A .
INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH, 1993, 32 (04) :709-715
[45]   RECOVERY OF URANIUM FROM SEAWATER .13. LONG-TERM STABILITY-TESTS FOR HIGH-PERFORMANCE CHELATING RESINS CONTAINING AMIDOXIME GROUPS AND EVALUATION OF ELUTION PROCESS [J].
EGAWA, H ;
KABAY, N ;
SHUTO, T ;
JYO, A .
INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH, 1993, 32 (03) :540-547
[46]   INFLUENCE OF CROSSLINKING AND POROSITY ON THE URANIUM ADSORPTION OF MACRORETICULAR CHELATING RESIN CONTAINING AMIDOXIME GROUPS [J].
EGAWA, H ;
NONAKA, T ;
NAKAYAMA, M .
JOURNAL OF MACROMOLECULAR SCIENCE-CHEMISTRY, 1988, A25 (10-11) :1407-1425
[47]   RECOVERY OF URANIUM FROM SEAWATER .12. PREPARATION AND CHARACTERIZATION OF LIGHTLY CROSS-LINKED HIGHLY POROUS CHELATING RESINS CONTAINING AMIDOXIME GROUPS [J].
EGAWA, H ;
KABAY, N ;
SHUTO, T ;
JYO, A .
JOURNAL OF APPLIED POLYMER SCIENCE, 1992, 46 (01) :129-142
[48]   Kinetics and thermodynamics of adsorption of trace amount of uranium on activated carbon [J].
El-Sayed, A. A. .
RADIOCHIMICA ACTA, 2008, 96 (08) :481-486
[49]   Sorption of uranium(VI) from aqueous solution onto magnesium silicate hollow spheres [J].
Fan, Fangli ;
Ding, Huajie ;
Bai, Jing ;
Wu, Xiaolei ;
Lei, Fuan ;
Tian, Wei ;
Wang, Yang ;
Qin, Zhi .
JOURNAL OF RADIOANALYTICAL AND NUCLEAR CHEMISTRY, 2011, 289 (02) :367-374
[50]   Adsorption of uranyl ion onto an anthraquinone based ion-imprinted copolymer [J].
Fasihi, J. ;
Alahyari, S. Ammari ;
Shamsipur, M. ;
Sharghi, H. ;
Charkhi, A. .
REACTIVE & FUNCTIONAL POLYMERS, 2011, 71 (08) :803-808