High-order harmonic generation by bi-elliptical orthogonally polarized two-color fields

被引:30
作者
Milosevic, D. B. [1 ,2 ,3 ]
Becker, W. [3 ,4 ]
机构
[1] Univ Sarajevo, Fac Sci, Zmaja Od Bosne 35, Sarajevo 71000, Bosnia & Herceg
[2] Acad Sci & Arts Bosnia & Herzegovina, Bistrik 7, Sarajevo 71000, Bosnia & Herceg
[3] Max Born Inst, Max Born Str 2a, D-12489 Berlin, Germany
[4] Natl Res Nucl Univ MEPhI, Kashirskoe Shosse 31, Moscow 115409, Russia
关键词
CIRCULAR-DICHROISM; ULTRAFAST DYNAMICS; LASER; IONIZATION; EMISSION; TIME; SPIN;
D O I
10.1103/PhysRevA.102.023107
中图分类号
O43 [光学];
学科分类号
070207 ; 0803 ;
摘要
Based on the strong-field approximation, we report results for high-order harmonic generation by bi-elliptical orthogonally polarized two-color (BEOTC) fields with frequency ratios of 2:1 and 3:1 and fundamental wavelengths of 800 and 1800 nm. A BEOTC field denotes the superposition of two copropagating counter-rotating elliptically polarized fields with different wavelengths and orthogonal semimajor axes. Its two limiting cases are the bicircular field and the linearly polarized orthogonal two-color field [D. B. Milosevic' and W. Becker, Phys. Rev. A 100, 031401(R) (2019)]. A detailed analysis of the high-order harmonic intensities and ellipticities as functions of the harmonic order, the ellipticity, and the relative phase between the two driving-field components is presented. Regions of the parameter space are identified where the harmonic ellipticities are very high. Surprisingly, this can be the case already for very small ellipticity (as small as epsilon = 0.01) of the driving field. This can be important for practical applications. In the opposite limit where the BEOTC field is close to bicircular, the selection rules that govern the latter case can also be very quickly invalidated. For the 2:1 case, this can result in an apparent shift of the selection rules by one harmonic order.
引用
收藏
页数:14
相关论文
共 69 条
[1]   Photoexcitation circular dichroism in chiral molecules [J].
Beaulieu, S. ;
Comby, A. ;
Descamps, D. ;
Fabre, B. ;
Garcia, G. A. ;
Geneaux, R. ;
Harvey, A. G. ;
Legare, F. ;
Masin, Z. ;
Nahon, L. ;
Ordonez, A. F. ;
Petit, S. ;
Pons, B. ;
Mairesse, Y. ;
Smirnova, O. ;
Blanchet, V. .
NATURE PHYSICS, 2018, 14 (05) :484-+
[2]   Probing ultrafast dynamics of chiral molecules using time-resolved photoelectron circular dichroism [J].
Beaulieu, Samuel ;
Comby, Antoine ;
Fabre, Baptiste ;
Descamps, Dominique ;
Ferre, Amelie ;
Garcia, Gustavo ;
Geneaux, Romain ;
Legare, Francois ;
Nahon, Laurent ;
Petit, Stephane ;
Ruchon, Thierry ;
Pons, Bernard ;
Blanchet, Valerie ;
Mairesse, Yann .
FARADAY DISCUSSIONS, 2016, 194 :325-348
[3]   Distinguishing the ultrafast dynamics of spin and orbital moments in solids [J].
Boeglin, C. ;
Beaurepaire, E. ;
Halte, V. ;
Lopez-Flores, V. ;
Stamm, C. ;
Pontius, N. ;
Duerr, H. A. ;
Bigot, J. -Y. .
NATURE, 2010, 465 (7297) :458-U78
[4]   Interlocked attosecond pulse trains in slightly bi-elliptical high harmonic generation [J].
Bordo, Eliyahu ;
Kfir, Ofer ;
Zayko, Sergey ;
Neufeld, Ofer ;
Fleischer, Avner ;
Ropers, Claus ;
Cohen, Oren .
JOURNAL OF PHYSICS-PHOTONICS, 2020, 2 (03)
[5]   Spectroscopy of atomic orbital sizes using bi-elliptical high-order harmonic generation [J].
Bordo, Eliyahu ;
Neufeld, Ofer ;
Kfir, Ofer ;
Fleischer, Avner ;
Cohen, Oren .
PHYSICAL REVIEW A, 2019, 100 (04)
[6]   Asymmetry in photoelectron emission from chiral molecules induced by circularly polarized light [J].
Böwering, N ;
Lischke, T ;
Schmidtke, B ;
Müller, N ;
Khalil, T ;
Heinzmann, U .
PHYSICAL REVIEW LETTERS, 2001, 86 (07) :1187-1190
[7]   Trajectory Selection in High Harmonic Generation by Controlling the Phase between Orthogonal Two-Color Fields [J].
Brugnera, Leonardo ;
Hoffmann, David J. ;
Siegel, Thomas ;
Frank, Felix ;
Zair, Amelle ;
Tisch, John W. G. ;
Marangos, Jonathan P. .
PHYSICAL REVIEW LETTERS, 2011, 107 (15)
[8]   Enhancement of high harmonics generated by field steering of electrons in a two-color orthogonally polarized laser field [J].
Brugnera, Leonardo ;
Frank, Felix ;
Hoffmann, David J. ;
Torres, Ricardo ;
Siegel, Thomas ;
Underwood, Jonathan G. ;
Springate, Emma ;
Froud, Chris ;
Turcu, Edmond I. C. ;
Tisch, John W. G. ;
Marangos, Jonathan P. .
OPTICS LETTERS, 2010, 35 (23) :3994-3996
[9]   Tomographic reconstruction of circularly polarized high-harmonic fields: 3D attosecond metrology [J].
Chen, Cong ;
Tao, Zhensheng ;
Hernandez-Garcia, Carlos ;
Matyba, Piotr ;
Carr, Adra ;
Knut, Ronny ;
Kfir, Ofer ;
Zusin, Dimitry ;
Gentry, Christian ;
Grychtol, Patrik ;
Cohen, Oren ;
Plaja, Luis ;
Becker, Andreas ;
Jaron-Becker, Agnieszka ;
Kapteyn, Henry ;
Murnane, Margaret .
SCIENCE ADVANCES, 2016, 2 (02)
[10]   EXPERIMENTAL CONFIRMATION OF THE X-RAY MAGNETIC CIRCULAR-DICHROISM SUM-RULES FOR IRON AND COBALT [J].
CHEN, CT ;
IDZERDA, YU ;
LIN, HJ ;
SMITH, NV ;
MEIGS, G ;
CHABAN, E ;
HO, GH ;
PELLEGRIN, E ;
SETTE, F .
PHYSICAL REVIEW LETTERS, 1995, 75 (01) :152-155