Impact ionization of molecular oxygen by 3.5-MeV/u bare carbon ions

被引:21
作者
Nandi, Saikat [1 ]
Agnihotri, Aditya N. [1 ]
Kasthurirangan, S. [2 ]
Kumar, Ajay [3 ]
Tachino, Carmen A. [4 ]
Rivarola, Roberto D. [4 ]
Martin, F. [5 ,6 ]
Tribedi, Lokesh C. [1 ]
机构
[1] Tata Inst Fundamental Res, Bombay 400005, Maharashtra, India
[2] Inst Chem Technol, Bombay 400019, Maharashtra, India
[3] Bhabha Atom Res Ctr, NPD, Bombay 400085, Maharashtra, India
[4] Univ Nacl Rosario, Inst Fis Rosario, CONICET, RA-2000 Rosario, Argentina
[5] Univ Autonoma Madrid, Dept Quim, E-28049 Madrid, Spain
[6] Inst Madrileno Estudios Avanzados Nanociencia, Madrid 28049, Spain
来源
PHYSICAL REVIEW A | 2012年 / 85卷 / 06期
关键词
ANGULAR-DISTRIBUTIONS; ELECTRON-EMISSION; GAUSSIAN EXPANSIONS; ENERGY ELECTRONS; ATOM COLLISIONS; HYDROGEN; INTERFERENCE; H+; HE;
D O I
10.1103/PhysRevA.85.062705
中图分类号
O43 [光学];
学科分类号
070207 ; 0803 ;
摘要
We have measured the absolute double-differential cross sections (DDCSs) for electron emission in ionization of O-2 molecules under the impact of 3.5-MeV/u C6+ ions. The data were collected between 10 and 600 eV, in an angular range of 30 degrees. to 150 degrees. The single-differential cross sections (SDCSs) in emission angle and electron energy are deduced from the electron DDCS spectra. Also, the total cross section has been obtained from the SDCS spectra. The DDCS spectra as well as the SDCS spectra are compared with continuum distorted-wave eikonal initial-state calculations which employ molecular wave functions built as linear combinations of atomic orbitals. The DDCS ratio i.e. sigma(O2)/2 sigma(O), derived by dividing the experimental DDCS for molecular oxygen with the theoretical DDCS for atomic oxygen, does not show any primary or secondary oscillations arising from Young-type interference, which is apparently in contrast to what has been observed earlier for H-2 and in agreement with the model calculation. Similarly, the forward-backward angular asymmetry increases monotonically with the velocity of the emitted electrons. However, the results on the DDCSs, SDCSs, the asymmetry parameter, and the nonexistence of oscillations are in qualitative agreement with the predictions of the model used.
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页数:8
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