NON-RESONANT TWO-PHOTON ABSORPTION CONTROL BY TWO TIME-DELAYED LASER PULSES

被引：3

作者：

Lu, Chenhui ^{[1
,2
]}

Zhang, Shian ^{[1
,2
]}

Jia, Tianqing ^{[1
,2
]}

Qiu, Jianrong ^{[3
,4
]}

Sun, Zhenrong ^{[1
,2
]}

机构：

[1] E China Normal Univ, State Key Lab Precis Spect, Shanghai 200062, Peoples R China

[2] E China Normal Univ, Dept Phys, Shanghai 200062, Peoples R China

[3] S China Univ Technol, State Key Lab Luminescent Mat & Devices, Guangzhou 510640, Guangdong, Peoples R China

[4] S China Univ Technol, Inst Opt Commun Mat, Guangzhou 510640, Guangdong, Peoples R China

来源：

JOURNAL OF NONLINEAR OPTICAL PHYSICS & MATERIALS | 2013年 / 22卷 / 01期

关键词：

Two-photon absorption; coherent control; FEMTOSECOND QUANTUM CONTROL; EXCITATION EFFICIENCY; COHERENT CONTROL; FLUORESCENCE; TRANSITIONS; PERYLENE; STORAGE;

D O I：

10.1142/S0218863513500082

中图分类号：

O43 [光学];

学科分类号：

070207 ; 0803 ;

摘要：

In this paper, we theoretically investigate the control of the non-resonant two-photon absorption induced by two time-delayed laser pulses, and an analytical solution for the dependence of the two-photon transition probability on the time delay and relative carrier-envelope phase of the two laser pulses is achieved. We show that the two-photon absorption can be significantly enhanced or completely suppressed by varying the time delay between the two laser pulses or their relative carrier-envelope phase. We also show that the two-photon absorption can be selectively excited when two excited states are simultaneously excited. Furthermore, we discuss the two-photon absorption control in the molecular system and analyze the effect of the absorption bandwidth on the control efficiency of the two-photon absorption.

引用

页数：9

共 25 条

[1] Photophysical characterization, two-photon absorption and optical power limiting of two fluorenylperylene diimides [J].

Belfield, Kevin A. ;

Bondar, Mykhailo V. ;

Hernandez, Florencio E. ;

Przhonska, Olga V. .

JOURNAL OF PHYSICAL CHEMISTRY C, 2008, 112 (14) :5618-5622

[2]

Bhawalkar J D, 1997, J Clin Laser Med Surg, V15, P201

[3] Temporal coherent control in two-photon transitions: From optical interferences to quantum interferences [J].

Blanchet, V ;

Nicole, C ;

Bouchene, MA ;

Girard, B .

PHYSICAL REVIEW LETTERS, 1997, 78 (14) :2716-2719

[4] Liquid-phase adaptive femtosecond quantum control: Removing intrinsic intensity dependencies [J].

Brixner, T ;

Damrauer, NH ;

Kiefer, B ;

Gerber, G .

JOURNAL OF CHEMICAL PHYSICS, 2003, 118 (08) :3692-3701

[5] Femtosecond polarization pulse shaping [J].

Brixner, T ;

Gerber, G .

OPTICS LETTERS, 2001, 26 (08) :557-559

[6] Enhancement of intermediate-field two-photon absorption by rationally shaped femtosecond pulses [J].

Chuntonov, Lev ;

Rybak, Leonid ;

Gandman, Andrey ;

Amitay, Zohar .

PHYSICAL REVIEW A, 2008, 77 (02)

[7] Two-photon polymerization initiators for three-dimensional optical data storage and microfabrication [J].

Cumpston, BH ;

Ananthavel, SP ;

Barlow, S ;

Dyer, DL ;

Ehrlich, JE ;

Erskine, LL ;

Heikal, AA ;

Kuebler, SM ;

Lee, IYS ;

McCord-Maughon, D ;

Qin, JQ ;

Röckel, H ;

Rumi, M ;

Wu, XL ;

Marder, SR ;

Perry, JW .

NATURE, 1999, 398 (6722) :51-54

[8] Two photon absorption and coherent control with broadband down-converted light [J].

Dayan, B ;

Pe'er, A ;

Friesem, AA ;

Silberberg, Y .

PHYSICAL REVIEW LETTERS, 2004, 93 (02) :023005-1

[9] 2-PHOTON LASER SCANNING FLUORESCENCE MICROSCOPY [J].

DENK, W ;

STRICKLER, JH ;

WEBB, WW .

SCIENCE, 1990, 248 (4951) :73-76

[10] Two-Photon Three-Dimensional Optical Storage Memory [J].

Dvornikov, A. S. ;

Walker, E. P. ;

Rentzepis, P. M. .

JOURNAL OF PHYSICAL CHEMISTRY A, 2009, 113 (49) :13633-13644

← 1 2 3 →