A microporous aluminum-based metal-organic framework for high methane, hydrogen, and carbon dioxide storage

被引：74

作者：

Wang, Bin ^{[1
,2
]}

Zhang, Xin ^{[2
]}

Huang, Hongliang ^{[4
]}

Zhang, Zhangjing ^{[1
]}

Yildirim, Taner ^{[3
]}

Zhou, Wei ^{[3
]}

Xiang, Shengchang ^{[1
]}

Chen, Banglin ^{[2
]}

机构：

[1] Fujian Normal Univ, Coll Chem & Mat Sci, Fujian Prov Key Lab Polymer Mat, 32 Shangsan Rd, Fuzhou 350007, Peoples R China

[2] Univ Texas San Antonio, Dept Chem, One UTSA Circle, San Antonio, TX 78249 USA

[3] NIST, Ctr Neutron Res, Gaithersburg, MD 20899 USA

[4] Tianjin Polytech Univ, State Key Lab Separat Membranes & Membrane Proc, Tianjin 300387, Peoples R China

来源：

NANO RESEARCH | 2021年 / 14卷 / 02期

基金：

中国博士后科学基金; 中国国家自然科学基金;

关键词：

metal-organic frameworks (MOFs); gas storage; methane; hydrogen; carbon dioxide; GAS-ADSORPTION; CAPTURE; CAPACITY; DESIGN;

D O I：

10.1007/s12274-020-2713-0

中图分类号：

O64 [物理化学（理论化学）、化学物理学];

学科分类号：

070304 ; 081704 ;

摘要：

We report a microporous aluminum-based metal-organic framework (MOF), BUT-22 for high methane (CH4), hydrogen (H-2), and carbon dioxide (CO2) storage. At 296 K and 80 bar, BUT-22 exhibits a high gravimetric CH(4)storage capacity of 530 cm(3)(STP)/g (0.379 g/g). BUT-22 also has a high gravimetric H(2)storage capacity of 12 wt.% at 100 bar and 77 K. In addition, the CO(2)adsorption studies revealed that BUT-22 exhibits a high absolute gravimetric CO(2)uptake of 1.7 g/g at 296 K and 40 bar.

引用

页码：507 / 511

页数：5

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