Role of fluid-density correlations in hydrodynamics: a multiparticle collision dynamics simulation study

被引:6
作者
Belushkin, M. [1 ]
Winkler, R. G. [2 ]
Foffi, G. [1 ]
机构
[1] Ecole Polytech Fed Lausanne, Inst Theoret Phys, CH-1015 Lausanne, Switzerland
[2] Forschungszentrum Julich, Inst Adv Simulat, Theoret Soft Matter & Biophys, D-52425 Julich, Germany
基金
瑞士国家科学基金会;
关键词
VELOCITY AUTOCORRELATION FUNCTION; VISCOUS COMPRESSIBLE FLUID; BROWNIAN-MOTION; DILUTE-SOLUTION; COMPLEX FLUIDS; BACKTRACKING; PROPAGATION; DIFFUSION; SOLVENT; SPHERE;
D O I
10.1039/c2sm26107c
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
Hydrodynamic interactions play a pivotal role in the dynamical behaviour of mesoscale systems such as colloidal suspensions, yet isolating their contribution from other effects remains a key challenge. Hydrodynamic correlations within a fluid are a consequence of local momentum conservation. Hence, as is commonly believed, violation of local momentum conservation should lead to non-hydrodynamic behaviour, where long-range correlations in the fluid are absent. Here, we demonstrate that generally this is a necessary but not sufficient criterion to achieve non-hydrodynamic behaviour. The motion of a massive particle leads to density modulations within the fluid. When the mechanisms underlying the relaxation processes of such modulations are removed, the dynamical behaviour of the system becomes unphysical. We show how the density relaxation mechanisms can be reintroduced in multiparticle collision dynamics (MPC) simulations, providing a consistent description of a system without hydrodynamic interactions.
引用
收藏
页码:9886 / 9891
页数:6
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