Unexpected air pollution with marked emission reductions during the COVID-19 outbreak in China

被引:686
作者
Le, Tianhao [1 ]
Wang, Yuan [1 ]
Liu, Lang [2 ,3 ]
Yang, Jiani [1 ]
Yung, Yuk L. [1 ]
Li, Guohui [2 ,3 ]
Seinfeld, John H. [4 ,5 ]
机构
[1] CALTECH, Div Geol & Planetary Sci, Pasadena, CA 91125 USA
[2] Chinese Acad Sci, Inst Earth Environm, State Key Lab Loess & Quaternary Geol, Xian, Shaanxi, Peoples R China
[3] Chinese Acad Sci, Inst Earth Environm, Key Lab Aerosol Chem & Phys, Xian, Shaanxi, Peoples R China
[4] CALTECH, Div Chem & Chem Engn, Pasadena, CA 91125 USA
[5] CALTECH, Div Engn & Appl Sci, Pasadena, CA 91125 USA
关键词
MEXICO-CITY; MODELING SYSTEM; APEC BLUE; AEROSOLS; HAZE; HONO; PHOTOCHEMISTRY; GASES;
D O I
10.1126/science.abb7431
中图分类号
O [数理科学和化学]; P [天文学、地球科学]; Q [生物科学]; N [自然科学总论];
学科分类号
07 ; 0710 ; 09 ;
摘要
The absence of motor vehicle traffic and suspended manufacturing during the coronavirus disease 2019 (COVID-19) pandemic in China enabled assessment of the efficiency of air pollution mitigation. Up to 90% reduction of certain emissions during the city-lockdown period can be identified from satellite and ground-based observations. Unexpectedly, extreme particulate matter levels simultaneously occurred in northern China. Our synergistic observation analyses and model simulations show that anomalously high humidity promoted aerosol heterogeneous chemistry, along with stagnant airflow and uninterrupted emissions from power plants and petrochemical facilities, contributing to severe haze formation. Also, because of nonlinear production chemistry and titration of ozone in winter, reduced nitrogen oxides resulted in ozone enhancement in urban areas, further increasing the atmospheric oxidizing capacity and facilitating secondary aerosol formation.
引用
收藏
页码:702 / +
页数:26
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