Depth resolved studies of SrTiO3 defects using x-ray excited optical luminescence and cathodoluminescence

被引:9
作者
Rosenberg, R. A. [1 ]
Choi, Y. [1 ]
Vijayalakshmi, K. [1 ]
Kareev, M. [2 ]
Tchakhalian, J. [2 ]
Balaz, Snjezana [3 ,4 ]
Brillson, L. J. [3 ,4 ]
机构
[1] Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA
[2] Univ Arkansas, Dept Phys, Fayetteville, AR 72701 USA
[3] Ohio State Univ, Dept Elect & Comp Engn, Columbus, OH 43210 USA
[4] Ohio State Univ, Dept Phys, Columbus, OH 43210 USA
基金
美国国家科学基金会;
关键词
CRYOGENIC TEMPERATURES; DIELECTRIC-PROPERTIES; GALLIUM-ARSENIDE; PHOTOLUMINESCENCE; GAN; EXCITATION; FILMS; SPECTROSCOPY; DEPENDENCE; INTERFACES;
D O I
10.1063/1.4807117
中图分类号
O59 [应用物理学];
学科分类号
摘要
We have performed comparative depth-dependent x-ray excited optical luminescence (XEOL) and depth resolved cathodoluminescence spectroscopy measurements in order to understand the native point defect distribution in three SrTiO3 samples. Both techniques found surface segregation of Ti3+ defects, but apparent differences in the oxygen vacancy distribution. Due to the lower excitation flux densities employed in XEOL, there is a delayed onset ("dead layer") revealed in the oxygen defect depth distribution, which results from band bending near the surface. By modeling the data, we are able to estimate the Ti3+ depth distribution and the depletion layer width. (C) 2013 AIP Publishing LLC.
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页数:5
相关论文
共 44 条
[1]  
Addiss J. R. R., 1968, APPL PHYS LETT, V12, P397
[2]   Dependence of GaN photoluminescence on the excitation intensity [J].
Bessolov, VN ;
Evstropov, VV ;
Kompan, ME ;
Mesh, MV .
SEMICONDUCTORS, 2002, 36 (10) :1128-1131
[3]   Nanoscale luminescence spectroscopy of defects at buried interfaces and ultrathin films [J].
Brillson, LJ .
JOURNAL OF VACUUM SCIENCE & TECHNOLOGY B, 2001, 19 (05) :1762-1768
[4]   Magnetic effects at the interface between non-magnetic oxides [J].
Brinkman, A. ;
Huijben, M. ;
Van Zalk, M. ;
Huijben, J. ;
Zeitler, U. ;
Maan, J. C. ;
Van der Wiel, W. G. ;
Rijnders, G. ;
Blank, D. H. A. ;
Hilgenkamp, H. .
NATURE MATERIALS, 2007, 6 (07) :493-496
[5]  
Casey J. H. C., 1971, J APPL PHYS, V42, P2774
[6]   METHOD FOR THE ANALYSIS OF SATURATION EFFECTS OF CATHODOLUMINESCENCE IN PHOSPHORS - APPLIED TO ZN2SIO4-MN AND Y3AL5O12-TB [J].
DELEEUW, DM ;
THOOFT, GW .
JOURNAL OF LUMINESCENCE, 1983, 28 (03) :275-300
[7]   SATURATION AND VOLTAGE EFFECTS IN CATHODOLUMINESCENCE [J].
DOWLING, PH ;
SEWELL, JR .
JOURNAL OF THE ELECTROCHEMICAL SOCIETY, 1953, 100 (01) :22-33
[8]   OPTICAL-LUMINESCENCE YIELD SPECTRA PRODUCED BY X-RAY-EXCITATION [J].
EMURA, S ;
MORIGA, T ;
TAKIZAWA, J ;
NOMURA, M ;
BAUCHSPIESS, KR ;
MURATA, T ;
HARADA, K ;
MAEDA, H .
PHYSICAL REVIEW B, 1993, 47 (12) :6918-6930
[9]   Microwave dielectric properties of single-crystal quantum paraelectrics KTaO3 and SrTiO3 at cryogenic temperatures -: art. no. 104111 [J].
Geyer, RG ;
Riddle, B ;
Krupka, J ;
Boatner, LA .
JOURNAL OF APPLIED PHYSICS, 2005, 97 (10)
[10]   PHOTOELECTRONIC PROCESSES IN RUTILE [J].
GHOSH, AK ;
WAKIM, FG ;
ADDISS, RR .
PHYSICAL REVIEW, 1969, 184 (03) :979-&