Ammonia emissions from paddy fields are underestimated in China

被引:105
作者
Wang, Hongyuan [1 ]
Zhang, Dan [1 ]
Zhang, Yitao [1 ]
Zhai, Limei [1 ]
Yin, Bin [2 ]
Zhou, Feng [3 ]
Geng, Yucong [1 ]
Pan, Junting [1 ]
Luo, Jiafa [4 ]
Gu, Baojing [5 ]
Liu, Hongbin [1 ]
机构
[1] Chinese Acad Agr Sci, Inst Agr Resources & Reg Planning, Key Lab Nonpoint Source Pollut Control, Minist Agr, 12 Zhongguancun South St, Beijing 100081, Peoples R China
[2] Chinese Acad Sci, Inst Soil Sci, State Key Lab Soil & Sustainable Agr, Nanjing 210008, Jiangsu, Peoples R China
[3] Peking Univ, Sinofrance Inst Earth Syst Sci, Inst Integrated Watershed Management, Coll Urban & Environm Sci,Lab Earth Surface Proc, Beijing 100871, Peoples R China
[4] AgResearch, Ruakura Res Ctr, 10 Bisley Rd, Hamilton 3214, New Zealand
[5] Zhejiang Univ, Dept Land Management, Zijingang Campus,866 Yuhangtang Rd, Hangzhou 310058, Zhejiang, Peoples R China
基金
英国生物技术与生命科学研究理事会; 中国国家自然科学基金;
关键词
Nitrogen rate; Ammonia loss proportion; Non-linear response; Air pollution; Climate factor; NITROGEN USE EFFICIENCY; VOLATILIZATION LOSSES; MANAGEMENT-PRACTICES; CROPPING SYSTEM; RICE; NH3; INVENTORY; YIELD; EAST; UREA;
D O I
10.1016/j.envpol.2017.12.103
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
Excessive nitrogen (N) fertilizers are often used in China, and a large proportion of the N can be lost as ammonia (NH3). However, quantifying the NH3 emission from paddy fields is always affected by large uncertainties due to different measuring methods and other factors such as climate. In this study, using a standardized method, we measured the NH3 emissions in three typical annual rice cropping systems: single rice, double rice and rotation with other crops. The measurements were conducted for 2 years with a total of 3131 observations across China. Results showed that NH3 emissions accounted for 17.7% (14.4 -21.0%) of the N applied under current farm practice, which was 33.1% (10.6-52.6%) higher than previous estimates. Nitrogen application rate was the dominant factor influencing NH3 emission rate, which exponentially increased with the N fertilizer rate (p < .001). Total NH3 emissions from paddy fields were estimated at 1.7 Tg N yr(-1) in 2013 in China, several times the amount of N lost through leaching or runoff. This suggests that mitigation measures for non-point source pollution from cropland should take into account not only the N lost to water, but also to air, thereby improving air quality. (C) 2017 Elsevier Ltd. All rights reserved.
引用
收藏
页码:482 / 488
页数:7
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