Nonlinear spectroscopy with time- and frequency-gated photon counting: A superoperator diagrammatic approach

被引:22
作者
Dorfman, Konstantin E. [1 ]
Mukamel, Shaul [1 ]
机构
[1] Univ Calif Irvine, Irvine, CA 92697 USA
来源
PHYSICAL REVIEW A | 2012年 / 86卷 / 01期
基金
美国国家科学基金会;
关键词
FLUCTUATIONS; BEAMS;
D O I
10.1103/PhysRevA.86.013810
中图分类号
O43 [光学];
学科分类号
070207 ; 0803 ;
摘要
We present a diagrammatic technique for calculating quantum-detected nonlinear optical signals using loop diagrams that act in the joint matter plus field space. This formalism, which is based on time-ordered superoperators keeps track of the entangled matter plus field state, making it most suitable for spectroscopy applications. Photon counting is recast as a time and frequency convolution of a bare signal, which is given by a correlation function of matter, and a gating spectrogram.
引用
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页数:7
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