Enhanced ammonia response of Ti3C2Tx nanosheets supported by TiO2 nanoparticles at room temperature

被引:284
作者
Tai, Huiling [1 ]
Duan, Zaihua [1 ]
He, Zaizhou [1 ]
Li, Xian [2 ]
Xu, Jianglong [3 ]
Liu, Bohao [1 ]
Jiang, Yadong [1 ]
机构
[1] UESTC, Sch Optoelect Sci & Engn, State Key Lab Elect Thin Films & Integrated Devic, Chengdu 610054, Sichuan, Peoples R China
[2] Chinese Acad Agr Sci, Agr Informat Inst, Minist Agr, Key Lab Agr Informat Serv Technol, Beijing 100081, Peoples R China
[3] Soochow Univ, Jiangsu Key Lab Carbon Based Funct Mat & Devices, Inst Funct Nano & Soft Mat FUNSOM, Suzhou 215123, Peoples R China
关键词
Ti3C2Tx nanosheets; TiO2; nanoparticles; TiO2/Ti3C2Tx bilayer film; NH3 gas sensors; GAS SENSORS; 2-DIMENSIONAL TI3C2; OXIDE; SENSITIVITY;
D O I
10.1016/j.snb.2019.126874
中图分类号
O65 [分析化学];
学科分类号
070302 ; 081704 ;
摘要
As a novel 2D material, Ti3C2Tx has been proved to be promising in the field of room temperature ammonia (NH3) sensors by theoretical calculation and experimental testing. However, its NH3 sensing properties still need to be enhanced. In this short communication, the gas sensor based on TiO2/Ti3C2Tx bilayer film is fabricated for enhancing the NH3 sensing properties of pure Ti3C2Tx. The results show that the TiO2/Ti3C2Tx sensor exhibits larger response value (1.63 times) and shorter response/recovery times (0.65/0.52 times) that of pure Ti3C2Tx sensor to 10 ppm NH3 at room temperature of 25 degrees C (60.8% relative humidity). Meanwhile, the TiO2/Ti3C2Tx sensor is of good linear response (R-2 = 0.95596) at 2-10 ppm NH3 and can respond to NH3 as low as 0.5 ppm. This work is expected to provide useful reference for the development of high performance Ti3C2Tx-based NH3 sensors.
引用
收藏
页数:5
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