A series of resorcin [4] arene-based lanthanide-metal organic frameworks for barcode and luminescent multicolor tuning property

被引：17
|
作者：
Zhang, Hang [1 ]
Liu, Hui [1 ]
Jiang, Wei [2 ]
Zhao, Si-Si [1 ]
机构：
[1] Shenyang Normal Univ, Coll Chem & Chem Engn, Inst Catalysis Energy & Environm, Shenyang 110034, Liaoning, Peoples R China
[2] Jilin Normal Univ, Coll Environm Sci & Engn, Siping 136000, Peoples R China
来源：
DYES AND PIGMENTS | 2019年 / 171卷
基金：
中国国家自然科学基金;
关键词：
Lanthanide-metal organic frameworks; Octacarboxylate-functionalized resorcin[4] arene; Crystal structure; Barcode application; Luminescent multicolor tuning; COORDINATION POLYMERS; ENERGY-TRANSFER; HIGHLY LUMINESCENT; COLOR TUNABILITY; LIGAND; THERMOMETER; TB(III); EU(III); SYSTEMS; ACID;
D O I：
10.1016/j.dyepig.2019.107665
中图分类号：
O69 [应用化学];
学科分类号：
081704 ;
摘要：
Three lanthanide-metal organic frameworks, namely, [Ln(2)(H2L)(DMF)(2)(H2O2)(2)]center dot 4H(2)O[Ln = Tb (1); Eu (2); Gd (3)] have been prepared and structurally characterized. Isostructural Ln-MOFs (1)-(3) display unique 3D frameworks with (4(12).6(3)) topology. Remarkably, Ln-MOFs (1) and (2) show intense characteristic red and green emissions and long lifetimes thanks to the "antenna" linker of H2L6- anions. Codoped Eu/Tb-MOFs (4)-(12) were synthesized by varying the Eu3+:Tb3+ stoichiometry. More importantly, such codoped Eu/Tb-MOF material emits multiple emission colors by enhancement and quenching of different Ln(3+) centers, which could applied to potential barcode materials. In addition, by adjusting different excitation wavelengths, the luminescence control of codoped Eu/Tb-MOFs (4)-(12) is achieved.
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页数：8
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