High-resolution 129I bomb peak profile in an ice core from SE-Dome site, Greenland

被引:11
|
作者
Bautista, Angel T. [1 ,2 ]
Miyake, Yasuto [2 ]
Matsuzaki, Hiroyuki [2 ,3 ]
Iizuka, Yoshinori [4 ]
Horiuchi, Kazuho [5 ]
机构
[1] Philippine Nucl Res Inst, Dept Sci & Technol PNRI DOST, Commonwealth Ave, Quezon City 1101, Philippines
[2] Univ Tokyo, Dept Nucl Engn & Management, Bunkyo Ku, Tokyo 1138656, Japan
[3] Univ Tokyo, Univ Museum, Micro Anal Lab, Tandem Accelerator MALT,Bunkyo Ku, Tokyo 1130032, Japan
[4] Hokkaido Univ, Inst Low Temp Sci, Sapporo, Hokkaido 060098, Japan
[5] Hirosaki Univ, Grad Sch Sci & Technol, Hirosaki, Aomori 0368560, Japan
关键词
Iodine-129; Tritium; Nuclear weapons testing; Time marker; Environmental tracer; ATMOSPHERIC HT; NUCLEAR ACTIVITIES; MAJOR SOURCES; FUKUSHIMA; TRANSPORT; TRITIUM; DEPOSITION; RECORD; TIME;
D O I
10.1016/j.jenvrad.2017.12.015
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
I-129 in natural archives, such as ice cores, can be used as a proxy for human nuclear activities, age marker, and environmental tracer. Currently, there is only one published record of I-129 in ice core (i.e., from Fiescherhorn Glacier, Swiss Alps) and its limited time resolution (1-2 years) prevents the full use of I-129 for the mentioned applications. Here we show I-129 concentrations in an ice core from SE-Dome, Greenland, covering years 1956-1976 at a time resolution of similar to 6 months, the most detailed record to date. Results revealed I-129 bomb peaks in years 1959, 1962, and 1963, associated to tests performed by the former Soviet Union, one year prior, in its Novaya Zemlya test site. All I-129 bomb peaks were observed in winter (1958.9, 1962.1, and 1963.0), while tritium bomb peaks, another prominent radionuclide associated with nuclear bomb testing, were observed in spring or summer (1959.3, and 1963.6; Iizuka et al., 2017). These results indicate that I-129 bomb peaks can be used as annual and seasonal age markers for these years. Furthermore, we found that I-129 recorded nuclear fuel reprocessing signals and that these can be potentially used to correct timing of estimated I-129 releases during years 1964-1976. Comparisons with other published records of I-129 in natural archives showed that I-129 can be used as common age marker and tracer for different types of records. Most notably, the 1963 I-129 bomb peak can be used as common age marker for ice and coral cores, providing the means to reconcile age models and associated trends from the polar and tropical regions, respectively.
引用
收藏
页码:14 / 21
页数:8
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