Selective coherent control of the lifetime of a resonance state with laser pulses

被引:7
|
作者
Garcia-Vela, A. [1 ]
机构
[1] CSIC, Inst Fis Fundamental, Madrid 28006, Spain
来源
JOURNAL OF CHEMICAL PHYSICS | 2013年 / 139卷 / 13期
关键词
DISSOCIATION; NEBR2; DYNAMICS;
D O I
10.1063/1.4823983
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
It is shown that new possibilities for control of the lifetime of a system in a resonance state emerge when the density of resonances overlapping and interfering with the target resonance increases. When using a control scheme combining two pump laser pulses, it is found that increasing the density of resonance states overlapping with the target one increases the selectivity of the scheme applied, and leads to achieve a remarkably higher degree of control. Lifetime enhancements by factors up to 20 are obtained when this selectivity is applied. The underlying reasons for such strong enhancements are analyzed and explained in the light of the equations of the model applied. Application of this strategy to control and enhance the lifetime of a system in excited states is envisioned. (C) 2013 AIP Publishing LLC.
引用
收藏
页数:9
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