Selective coherent control of the lifetime of a resonance state with laser pulses

被引:7
|
作者
Garcia-Vela, A. [1 ]
机构
[1] CSIC, Inst Fis Fundamental, Madrid 28006, Spain
来源
JOURNAL OF CHEMICAL PHYSICS | 2013年 / 139卷 / 13期
关键词
DISSOCIATION; NEBR2; DYNAMICS;
D O I
10.1063/1.4823983
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
It is shown that new possibilities for control of the lifetime of a system in a resonance state emerge when the density of resonances overlapping and interfering with the target resonance increases. When using a control scheme combining two pump laser pulses, it is found that increasing the density of resonance states overlapping with the target one increases the selectivity of the scheme applied, and leads to achieve a remarkably higher degree of control. Lifetime enhancements by factors up to 20 are obtained when this selectivity is applied. The underlying reasons for such strong enhancements are analyzed and explained in the light of the equations of the model applied. Application of this strategy to control and enhance the lifetime of a system in excited states is envisioned. (C) 2013 AIP Publishing LLC.
引用
收藏
页数:9
相关论文
共 50 条
  • [1] Coherent control of a resonance lifetime with laser pulses
    Garcia-Vela, A.
    CHEMICAL PHYSICS LETTERS, 2013, 563 : 30 - 36
  • [2] Active control of the lifetime of excited resonance states by means of laser pulses
    Garcia-Vela, A.
    JOURNAL OF CHEMICAL PHYSICS, 2012, 136 (13):
  • [3] Strong Enhancement of the Lifetime of a Resonance State by Using a Combination of Two Laser Pulses
    Garcia-Vela, A.
    JOURNAL OF PHYSICAL CHEMISTRY LETTERS, 2012, 3 (15): : 1941 - 1945
  • [4] Coherent control with femtosecond laser pulses
    Baumert, T
    Helbing, J
    Gerber, G
    Woste, L
    Zewail, AH
    Troe, J
    Manz, J
    Kobayashi, T
    Letokhov, VS
    Even, U
    Chergui, M
    Neumark, DM
    Rice, SA
    CHEMICAL REACTIONS AND THEIR CONTROL ON THE FEMTOSECOND TIME SCALE XXTH SOLVAY CONFERENCE ON CHEMISTRY, 1997, 101 : 47 - 82
  • [5] Quantum coherent control of ultrashort laser pulses
    ZHOU JianYing
    Chinese Science Bulletin, 2008, (05) : 652 - 658
  • [6] Temporal compression of laser pulses by coherent control
    Tognetti, M. V.
    Buffa, R.
    Cavalieri, S.
    Fini, L.
    Ignesti, E.
    Saji, E.
    COMPUTATION IN MODERN SCIENCE AND ENGINEERING VOL 2, PTS A AND B, 2007, 2 : 829 - +
  • [7] Quantum coherent control of ultrashort laser pulses
    Zhou JianYing
    Zeng JianHua
    Li JunTao
    CHINESE SCIENCE BULLETIN, 2008, 53 (05): : 652 - 658
  • [8] Pump-dump coherent control with partially coherent laser pulses
    Jiang, XP
    Shapiro, M
    Brumer, P
    JOURNAL OF CHEMICAL PHYSICS, 1996, 104 (02): : 607 - 615
  • [9] Coherent control of atom ionization with sequential laser pulses
    Poluektov, NP
    Fedorov, MV
    LASER PHYSICS, 2002, 12 (04) : 769 - 774
  • [10] Coherent Pulse Stacking of Solid-State Laser Pulses
    Astrauskas, I.
    Kaksis, E.
    Floery, T.
    Andriukaitis, G.
    Pugzlys, A.
    Curilla, L.
    Baltuska, A.
    Ruppe, J.
    Chen, S.
    Galvanauskas, A.
    Balciunas, T.
    2016 CONFERENCE ON LASERS AND ELECTRO-OPTICS (CLEO), 2016,